王琛^1,,
张秀明²,
段佳堃¹,
赵占轻³,
遆超普⁴,
王贵师⁵,
周丰⁶,
张霖⁷,
刘宏斌⁸,
董红敏⁹,
朱志平⁹,
谷保静^1,,
1.浙江大学环境与资源学院　杭州　310058
2.墨尔本大学　墨尔本 VIC　3010
3.河北地质大学土地科学与空间规划学院　石家庄　050031
4.中国科学院南京土壤研究所　南京　210008
5.中国科学院合肥物质科学研究院　合肥　230031
6.北京大学城市与环境学院　北京　100871
7.北京大学物理学院　北京　100871
8.中国农业科学院农业资源与农业区划研究所　北京　100081
9.中国农业科学院农业环境与可持续发展研究所　北京　100081
基金项目:国家重点研发计划项目(2018YFC0213304)资助

详细信息

作者简介:王琛, 主要研究方向为农业氮循环。E-mail: wang.chen@zju.edu.cn

通讯作者:谷保静, 主要研究方向为氮循环及其调控、农业污染治理与绿色发展。E-mail: bjgu@zju.edu.cn

中图分类号:X511

计量

文章访问数:134
HTML全文浏览量:98
PDF下载量:65
被引次数:0

出版历程

收稿日期:2021-05-17
录用日期:2021-08-16
网络出版日期:2021-10-08
刊出日期:2021-12-09

A high-resolution ammonia emission inventory for cropland and livestock production in China

WANG Chen^1,,
ZHANG Xiuming²,
DUAN Jiakun¹,
ZHAO Zhanqing³,
TI Chaopu⁴,
WANG Guishi⁵,
ZHOU Feng⁶,
ZHANG Lin⁷,
LIU Hongbin⁸,
DONG Hongmin⁹,
ZHU Zhiping⁹,
GU Baojing^1,,
1. College of Environmental and Resource Sciences, Zhejiang University, Hangzhou 310058, China
2. The University of Melbourne, Melbourne, VIC 3010, Australia
3. School of Land Science and Space Planning, Hebei GEO University, Shijiazhuang 050031, China
4. Institute of Soil Science, Chinese Academy of Sciences, Nanjing 210008, China
5. Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei 230031, China
6. College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
7. School of Physics, Peking University, Beijing 100871, China
8. Institute of Agricultural Resources and Regional Planning, Chinese Academy of Agricultural Sciences, Beijing 100081, China
9. Institute of Environmental and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences, Beijing 100081, China
Funds:This study was supported by the National Key Research and Development Program of China (2018YFC0213304)

More Information

Corresponding author:E-mail: bjgu@zju.edu.cn

摘要
HTML全文
图(3)表(0)
参考文献(32)
相关文章
施引文献
资源附件(0)
访问统计

摘要
摘要:氨(NH₃)挥发对生态系统和人体健康都带来负面影响, 其中农畜牧业占NH₃挥发总量的90%左右, 农牧业NH₃挥发也意味着氮肥流失, 给农民带来经济负担。本文梳理了国家重点研发专项“农畜牧业氨排放污染高效控制技术”项目中课题4“农牧业氨排放清单编制及减排评估技术研究”的主要内容, 重点介绍农畜牧业动态高精度氨排放清单编制的主要研究进展。本课题构建了农田NH₃挥发基础参数集和农事活动数据集, 以及畜禽养殖全链条NH₃挥发的特征参数集和养殖活动数据集, 完成了2017年全国2853个县(市) 1 km空间分辨率农田氮肥和畜禽养殖氨排放清单。中国2017年农田氮肥NH₃排放量为3.6 Tg, 南方排放强度高于北方; 畜牧业NH₃排放量为5.0 Tg, 其中室内圈舍和粪肥农田施用阶段NH₃排放较高。华北和华南地区为主要的排放热点区, 排放季节集中在春季和初夏。通过基于高分辨率农事活动数据的排放清单, 进而应用GEOS-Chem大气化学模型评估各种减排情景带来的空气质量改变, 指导精准减排和示范, 同时对全国不同区域农业NH₃排放特征识别和本地化、精细化农牧业管理提供参考。
关键词:氨挥发/
畜牧业/
氮肥/
排放清单/
减排情景
Abstract:Ammonia (NH₃) volatilization has negative impacts on ecosystem and human health and NH₃ emission from cropland and livestock accounts for approximately 90% of the total NH₃ emission, which also indicates nitrogen fertilizer loss and brings economic burden to farmers. We presented the main contents of topic 4 ‘Research on Ammonia Emission Inventory Compilation and Reduction Assessment for Cropland and Livestock Production’ in National Key Research and Development Program ‘High Efficiency Control Technology for Ammonia Emission Pollution from Cropland and Livestock Production’ and mainly focused on the latest progress of dynamic high-resolution ammonia emission inventory for cropland and livestock. This project developed the basic characteristic parameters and agricultural activity data set of both cropland and livestock production, then compiled the 1 km-resolution cropland nitrogen fertilizer and livestock NH₃ emission inventory of 2853 cities at county level in 2017. The NH₃ emission of cropland nitrogen fertilizer in China was 3.6 Tg of which the emission intensity in South China was higher than that in the North China. The total NH₃ emission inventory of livestock was 5.0 Tg of which the NH₃ emission in housing and manure spreading stage was higher. The North China Plain and Guangdong are the main emission hotspots and the emission peak was concentrated in spring and early summer. The GEOS-Chem atmospheric chemistry model was used to evaluate the air quality changes caused by various emission reduction scenarios, to guide the emission reduction strategies in demonstration area as well as provide information to localized emission characteristics and the fine management of agriculture in different regions.
Key words:Ammonia emission/
Livestock/
Nitrogen fertilizer/
Emission inventory/
Emission scenarios

HTML全文


图1“农牧业氨排放清单编制及减排评估技术”课题研究技术路线
Figure1.Technical route of the project ‘Research on Ammonia Emission Inventory Compilation and Reduction Assessment for Cropland and Livestock Production’


下载: 全尺寸图片幻灯片


图22017年中国农畜牧业氨排放县级空间分布情况
Figure2.Spatial distribution of ammonia emissions from cropland and livestock production at county level in China in 2017


下载: 全尺寸图片幻灯片


图32017年中国农畜牧业氨排放月份变化
Figure3.Monthly variation of ammonia emission from cropland and livestock production in China in 2017


下载: 全尺寸图片幻灯片


参考文献(32)

[1]	GALLOWAY J N, TOWNSEND A R, ERISMAN J W, et al. Transformation of the nitrogen cycle: recent trends, questions, and potential solutions[J]. Science, 2008, 320(5878): 889?892 doi: 10.1126/science.1136674
[2]	GU B J, JU X T, CHANG J, et al. Integrated reactive nitrogen budgets and future trends in China[J]. Proceedings of the National Academy of Sciences of the United States of America, 2015, 112(28): 8792?8797 doi: 10.1073/pnas.1510211112
[3]	HUANG X, SONG Y, LI M M, et al. A high-resolution ammonia emission inventory in China[J]. Global Biogeochemical Cycles, 2012, DOI: 10.1029/2011gb004161
[4]	ZHANG L, CHEN Y F, ZHAO Y H, et al. Agricultural ammonia emissions in China: reconciling bottom-up and top-down estimates[J]. Atmospheric Chemistry and Physics, 2018, 18(1): 339?355 doi: 10.5194/acp-18-339-2018
[5]	KANG Y N, LIU M X, SONG Y, et al. High-resolution ammonia emissions inventories in China from 1980 to 2012[J]. Atmospheric Chemistry and Physics, 2016, 16(4): 2043?2058 doi: 10.5194/acp-16-2043-2016
[6]	XU P, KOLOUTSOU-VAKAKIS S, ROOD M J, et al. Projections of NH3 emissions from manure generated by livestock production in China to 2030 under six mitigation scenarios[J]. Science of the Total Environment, 2017, 607/608: 78?86 doi: 10.1016/j.scitotenv.2017.06.258
[7]	ZHANG X M, GU B J, VAN GRINSVEN H, et al. Societal benefits of halving agricultural ammonia emissions in China far exceed the abatement costs[J]. Nature Communications, 2020, 11: 4357 doi: 10.1038/s41467-020-18196-z
[8]	LI S Q, ZHENG X H, ZHANG W, et al. Modeling ammonia volatilization following the application of synthetic fertilizers to cultivated uplands with calcareous soils using an improved DNDC biogeochemistry model[J]. Science of the Total Environment, 2019, 660: 931?946 doi: 10.1016/j.scitotenv.2018.12.379
[9]	XU R T, TIAN H Q, PAN S F, et al. Global ammonia emissions from synthetic nitrogen fertilizer applications in agricultural systems: Empirical and process-based estimates and uncertainty[J]. Global Change Biology, 2019, 25(1): 314?326 doi: 10.1111/gcb.14499
[10]	FU X, WANG S X, RAN L M, et al. Estimating NH3 emissions from agricultural fertilizer application in China using the bi-directional CMAQ model coupled to an agro-ecosystem model[J]. Atmospheric Chemistry and Physics, 2015, 15(12): 6637?6649 doi: 10.5194/acp-15-6637-2015
[11]	ZHAN X Y, CHEN C, WANG Q H, et al. Improved Jayaweera-Mikkelsen model to quantify ammonia volatilization from rice paddy fields in China[J]. Environmental Science and Pollution Research, 2019, 26(8): 8136?8147 doi: 10.1007/s11356-019-04275-2
[12]	Intergovernmental Panel on Climate Change (IPCC). 2019 Refinement to the 2006 IPCC Guidelines for National Greenhouse Gas Inventories: Agriculture, Forestry and Other Land Use. https://www.ipcc.ch/report/2019-refinement-to-the-2006-ipcc-guidelines-for-national-greenhouse-gas-inventories/
[13]	ZHAN X Y, ADALIBIEKE W, CUI X Q, et al. Improved estimates of ammonia emissions from global croplands[J]. Environmental Science & Technology, 2021, 55(2): 1329?1338
[14]	TI C P, XIA L L, CHANG S X, et al. Potential for mitigating global agricultural ammonia emission: a meta-analysis[J]. Environmental Pollution, 2019, 245: 141?148 doi: 10.1016/j.envpol.2018.10.124
[15]	ZHANG Y S, LUAN S J, CHEN L L, et al. Estimating the volatilization of ammonia from synthetic nitrogenous fertilizers used in China[J]. Journal of Environmental Management, 2011, 92(3): 480?493 doi: 10.1016/j.jenvman.2010.09.018
[16]	XU P, LIAO Y J, LIN Y H, et al. High-resolution inventory of ammonia emissions from agricultural fertilizer in China from 1978 to 2008[J]. Atmospheric Chemistry and Physics, 2016, 16(3): 1207?1218 doi: 10.5194/acp-16-1207-2016
[17]	XU P, ZHANG Y S, GONG W W, et al. An inventory of the emission of ammonia from agricultural fertilizer application in China for 2010 and its high-resolution spatial distribution[J]. Atmospheric Environment, 2015, 115: 141?148 doi: 10.1016/j.atmosenv.2015.05.020
[18]	董艳强, 陈长虹, 黄成, 等. 长江三角洲地区人为源氨排放清单及分布特征[J]. 环境科学学报, 2009, 29(8): 1611?1617 doi: 10.3321/j.issn:0253-2468.2009.08.005 DONG Y Q, CHEN C H, HUANG C, et al. Anthropogenic emissions and distribution of ammonia over the Yangtze River Delta[J]. Acta Scientiae Circumstantiae, 2009, 29(8): 1611?1617 doi: 10.3321/j.issn:0253-2468.2009.08.005
[19]	ZHENG J Y, YIN S S, KANG D W, et al. Development and uncertainty analysis of a high-resolution NH3 emissions inventory and its implications with precipitation over the Pearl River Delta region, China[J]. Atmospheric Chemistry and Physics, 2012, 12(15): 7041?7058 doi: 10.5194/acp-12-7041-2012
[20]	ZHOU Y, CHENG S Y, LANG J L, et al. A comprehensive ammonia emission inventory with high-resolution and its evaluation in the Beijing-Tianjin-Hebei (BTH) region, China[J]. Atmospheric Environment, 2015, 106: 305?317 doi: 10.1016/j.atmosenv.2015.01.069
[21]	WANG C, YIN S S, BAI L, et al. High-resolution ammonia emission inventories with comprehensive analysis and evaluation in Henan, China, 2006?2016[J]. Atmospheric Environment, 2018, 193: 11?23 doi: 10.1016/j.atmosenv.2018.08.063
[22]	WU S P, ZHANG Y J, SCHWAB J J, et al. High-resolution ammonia emissions inventories in Fujian, China, 2009?2015[J]. Atmospheric Environment, 2017, 162: 100?114 doi: 10.1016/j.atmosenv.2017.04.027
[23]	冯小琼, 陈军辉, 姜涛, 等. 四川省2005—2014年农业源氨排放清单及分布特征[J]. 环境科学, 2017, 38(7): 2728?2737 FENG X Q, CHEN J H, JIANG T, et al. Agricultural ammonia emission inventory and its spatial distribution in Sichuan Province from 2005 to 2014[J]. Environmental Science, 2017, 38(7): 2728?2737
[24]	杨志鹏. 基于物质流方法的中国畜牧业氨排放估算及区域比较研究[D]. 北京: 北京大学, 2008 YANG Z P. Estimation of ammonia emission from livestock in China based on mass-flow method and regional comparison[D]. Beijing: Peking University, 2008
[25]	刘东. 中国猪和奶牛粪尿氨(NH3)挥发的评价研究[D]. 保定: 河北农业大学, 2007 LIU D. Evaluation of NH3 emission from pig and dairy cow manure in China[D]. Baoding: Hebei Agricultural University, 2007
[26]	MA L, MA W Q, VELTHOF G L, et al. Modeling nutrient flows in the food chain of China[J]. Journal of Environmental Quality, 2010, 39(4): 1279?1289 doi: 10.2134/jeq2009.0403
[27]	廖仁郡, 陈玉成. 重庆市规模化畜禽养殖氨排放特征及减排策略研究[J]. 中国生态农业学报, 2017, 25(5): 769?777 LIAO R J, CHEN Y C. Characteristics of ammonia emission from large-scale livestock/poultry breeding and its mitigation countermeasures in Chongqing[J]. Chinese Journal of Eco-Agriculture, 2017, 25(5): 769?777
[28]	刘波, 童仪, 李安, 等. 长江三角洲地区畜禽养殖业氨排放清单研究[J]. 生态与农村环境学报, 2018, 34(11): 1042?1049 doi: 10.11934/j.issn.1673-4831.2018.11.012 LIU B, TONG Y, LI A, et al. Study on ammonia emission inventory of livestock over Yangtze River Delta[J]. Journal of Ecology and Rural Environment, 2018, 34(11): 1042?1049 doi: 10.11934/j.issn.1673-4831.2018.11.012
[29]	朱志平, 董红敏, 魏莎, 等. 中国畜禽粪便管理变化对温室气体排放的影响[J]. 农业环境科学学报, 2020, 39(4): 743?748 doi: 10.11654/jaes.2020-0095 ZHU Z P, DONG H M, WEI S, et al. Impact of changes in livestock manure management on greenhouse gas emissions in China[J]. Journal of Agro-Environment Science, 2020, 39(4): 743?748 doi: 10.11654/jaes.2020-0095
[30]	WU H, LI Y P, XIE Z H, et al. Estimating ammonia emissions from cropland in China based on the establishment of agro-region-specific models[J]. Agricultural and Forest Meteorology, 2021, 303: 108373 doi: 10.1016/j.agrformet.2021.108373
[31]	WANG C, CHENG K, REN C C, et al. An empirical model to estimate ammonia emission from cropland fertilization in China[J]. Environmental Pollution, 2021: 117982
[32]	ZHANG X M, REN C C, GU B J, et al. Uncertainty of nitrogen budget in China[J]. Environmental Pollution, 2021, 286: 117216 doi: 10.1016/j.envpol.2021.117216