1.Shandong Provincial Engineering and Technical Center of Light Manipulations, Shandong Provincial Key Laboratory of Optics and Photonic Device, School of Physics and Electronics, Shandong Normal University, Jinan 250358, China 2.Collaborative Innovation Center of Light Manipulations and Applications, Shandong Normal University, Jinan 250358, China 3.CAS Key Laboratory of Transparent and Opto-Functional Inorganic Materials, Synthetic Single Crystal Research Center, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 201899, China 4.College of Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
Fund Project:Project supported by the National Natural Science Foundation of China (Grant Nos. 11974220, 61635012, 61675135)
Received Date:05 March 2020
Accepted Date:14 March 2020
Available Online:23 March 2020
Published Online:20 September 2020
Abstract:As a new two-dimensional material, bismuth nanosheet is an effective modulator for realizing a mid-infrared pulsed laser, which benefits from its suitable band gap, higher carrier mobility and better room temperature stability, as well as its excellent electrical and optical properties. The mid-infrared single-crystal fiber is a preferable gain medium for high-power laser because of its advantages of both crystal and fiber. In this paper, a bismuth nanosheet saturable absorber is successfully prepared by the ultrasonic method and used for the first time in a diode-pumped Er:CaF2 single-crystal fiber mid-infrared passively Q-switching pulsed laser. A compact concave planar linear resonator is designed to study the Q-switching Er:CaF2 single-crystal fiber laser with bismuth nanosheets serving as saturable absorbers. The pump source is a fiber-coupled semiconductor laser with a core diameter of 105 μm, a numerical aperture of 0.22, and a central emission wavelength of 976 nm. The pump light is focused onto the front end of the gain medium through a coupled collimating system with a coupling ratio of 1∶2. The gain medium is a 4 at.% Er3+:CaF2 single-crystal fiber grown by the temperature gradient method, and this fiber has two polished but not coated ends, a diameter of 1.9 mm, and a length of 10 mm. To reduce the thermal effect, the single-crystal fiber is tightly wrapped with indium foil and mounted on a copper block with a constant temperature of 12 ℃. The input mirror has a high reflection coating at 2.7–2.95 μm and an antireflection coating at 974 nm, with a curvature radius of 100 mm. A group of partially transmitting plane mirrors are used as output couplers, respectively, with transmittances of 1%, 3%, and 5% at 2.7–2.95 μm. The total length of the resonant cavity is 26 mm. By inserting the bismuth nanosheet into the resonator and carefully adjusting its position and angle, a stable mid-infrared Q-switching laser is obtained. At the absorbed pump power of 1.52 W, a pulsed laser with an average output power of 190 mW is obtained for an output mirror with a transmittance of 3%. The shortest pulse width is 607 ns, the repetition frequency is 58.51 kHz, and the corresponding single pulse energy and peak power are 3.25 μJ and 5.35 W, respectively. Keywords:passively Q-switching laser/ mid-infrared laser/ bismuth nanosheets/ single-crystal fiber
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3.1.中红外单晶光纤的连续激光特性
首先研究了Er:CaF2单晶光纤的连续激光特性. Er:CaF2单晶光纤对976 nm抽运光的吸收率为77.3%. 激光输出功率随吸收抽运功率的变化如图2所示. 输出镜的透过率分别选用T = 1%, T = 3%和T = 5%时, 对应的吸收抽运阈值功率分别为0.12 W, 0.18 W和0.34 W. 当选用T = 3%的输出镜, 吸收抽运功率约为3.1 W时, 获得Er:CaF2单晶光纤的最大输出激光功率为0.94 W, 激光斜效率为32.0%. 连续激光的光谱如图3所示, 使用1%, 3%和5%透过率的输出镜, 获得的激光波长分别为2797.38 nm, 2751.65 nm和2758.90 nm. 图 2 连续激光输出功率随吸收抽运功率的变化 Figure2. Continuous-wave (CW) output power versus the absorbed pump power.
表1吸收抽运功率1.52 W时, 不同透过率下的调Q激光特性 Table1.Q-switched laser characteristics at the absorption pump power of 1.52 W
图 5 Er:CaF2单晶光纤Bi-NSs被动调Q激光(a)脉冲宽度、(b)重复频率、(c)单脉冲能量、(d)峰值功率随吸收抽运光的变化 Figure5. (a) Pulse duration, (b) repetition rate, (c) single pulse energy, and (d) peak power versus the absorbed pump power.