删除或更新信息,请邮件至freekaoyan#163.com(#换成@)

宁夏村镇饮用水中重金属暴露健康风险评估及不确定性分析

本站小编 Free考研考试/2021-12-30

朱美霖1,
杨晓莉2,
赵建明2,
于永军2,
田锋2,
朱新忠3,,
1. 宁夏医科大学基础医学院, 银川 750004;
2. 宁夏医科大学临床医学院, 银川 750004;
3. 宁夏农林科学院固原分院, 草畜资源开发与利用研究中心, 固原 756000
作者简介: 朱美霖(1987-),女,副教授,研究方向为环境中危险化学物质的健康危害,E-mail:jay70281@163.com.
通讯作者: 朱新忠,zhuxinzhong1962@163.com
基金项目: 国家自然科学基金资助项目(21667023);宁夏回族自治区重点研发计划项目(2019BFG02020);宁夏卫生计生委科研项目(2016-NW-006)


中图分类号: X171.5


Health Risk Assessment and Uncertainty Analysis Based on Heavy Metals Exposure by Drinking Water in Ningxia Rural Areas

Zhu Meilin1,
Yang Xiaoli2,
Zhao Jianming2,
Yu Yongjun2,
Tian Feng2,
Zhu Xinzhong3,,
1. College of Basic Medical Sciences, Ningxia Medical University, Yinchuan 750004, China;
2. Clinical College, Ningxia Medical University, Yinchuan 750004, China;
3. Research Center of Development and Utilization of Grass and Livestock Resources, Ningxia Academy of Agriculture and Forestry Sciences Guyuan Branch, Guyuan 756000, China
Corresponding author: Zhu Xinzhong,zhuxinzhong1962@163.com

CLC number: X171.5

-->

摘要
HTML全文
(0)(0)
参考文献(25)
相关文章
施引文献
资源附件(0)
访问统计

摘要:确定宁夏农村饮用水中重金属浓度,对保障宁夏居民饮水健康具有重要的意义。通过对宁夏回族自治区5个村镇饮用水采样调研,采用电感耦合等离子体-原子发射光谱(ICP-AES)法分析饮用水中5种常见重金属(砷、铬、镉、铅和铜)的浓度,并与我国《生活饮用水卫生标准》相比较,计算超标率;通过健康风险评估模型系统评价居民基于重金属污染的健康风险,进一步通过不确定性分析风险概率及敏感性。结果表明,5个采样点饮用水中砷元素均有超标现象(超标率<20%),其他4种重金属均未超标;5个样点饮用水中重金属单独暴露或共同暴露均不产生非致癌风险,但是砷元素所引起的致癌风险均超过美国环境保护局(US EPA)推荐的最大可接受风险水平10-4;不确定性分析中,概率评估结果显示对>90%的居民不存在非致癌风险,而对50%以上居民的致癌风险大于最大可接受风险水平;敏感性分析结果显示,非致癌风险中砷浓度和日摄入量为最敏感的2个参数,而致癌风险中砷浓度为最敏感参数。
关键词: 重金属/
饮用水/
健康风险/
不确定性分析/
概率评估

Abstract:Determining the heavy metal concentration of drinking water in Ningxia rural areas is of significance in ensuring drinking water security for inhabitants. In this study, we collected drinking water from five different villages and analyzed the concentrations of five common heavy metals (arsenic, chromium, cadmium, lead and copper) using inductively coupled plasma-atomic emission spectrometry (ICP-AES) method. Exceeding ratio was calculated by comparing with "hygienic standard for drinking water" in China. Based on health risk model, health risk was evaluated, and probability assessment and sensitivity analysis were taken by uncertainty analysis. Results showed that arsenic concentrations of less than 20% of the samples in five sampling sites exceeded the standard, while the concentrations of other four heavy metals not. The five metals could not cause obvious non-carcinogenic risk in each sampling site no matter individual risk or combined risk, while arsenic could increase carcinogenic risk due to its risk value over the maximum acceptable level set by United States Environmental Protection Agency (US EPA) (10-4). In uncertainty analysis, probability assessment results indicated that more than 90% of the population had no non-carcinogenic risk, but more than 50% of residents might have carcinogenic risk which exceeded the acceptable level; sensitivity analysis results suggested arsenic concentration and daily intake were the most sensitive factors in non-carcinogenic risk, and arsenic concentration was the key factor in carcinogenic risk.
Key words:heavy metals/
drinking water/
health risk/
uncertainty analysis/
probability assessment.

加载中
李仰斌, 张国华, 谢崇宝. 我国农村饮用水源现状及相关保护对策建议[J]. 中国农村水利水电, 2007, 11(1):1-4Li Y B, Zhang G H, Xie C B. Current situation and corresponding protection proposals of rural drinking water source in China[J]. China Rural Water and Hydropower, 2007, 11(1):1-4(in Chinese)
中华人民共和国卫生部, 中国国家标准管理委员会. 生活饮用水卫生标准GB5749-2006[S]. 北京:中华人民共和国卫生部, 中国国家标准管理委员会, 2006
齐拓野, 米文宝. 宁夏能源矿产资源的开发与利用[J]. 宁夏工程技术, 2006, 5(2):201-205Qi T Y, Mi W B. Study on exploitation and using of energy mineral resources in Ningxia[J]. Ningxia Engineering Technology, 2006, 5(2):201-205(in Chinese)
吴立新, 侯恩科. 西北五省(区)矿产资源开发与水资源保护对策[J]. 西安科技学院学报, 2000, 20(suppl.):63-67 Wu L X, Hou E K. Strategy on the development of mineral resources and the protection of water resource in the northwest area of China[J]. Journal of Xi'an University of Science & Technology, 2000, 20(suppl.):63-67(in Chinese)
戴向前, 刘昌明, 李丽娟. 我国农村饮水安全问题探讨与对策[J]. 地理学报, 2007, 9(62):907-916Dai X Q, Liu C M, Li L J. Discussion and countermeasures on safe drinking water in the rural areas of China[J]. Acta Geographica Sinica, 2007, 9(62):907-916(in Chinese)
高继军, 张力平, 黄圣彪, 等. 北京市饮用水源水重金属污染物健康风险的初步评价[J]. 环境科学, 2004, 25(2):47-50Gao J J, Zhang L P, Huang S B, et al. Preliminary health risk assessment of heavy metal in drinking water[J]. Environmental Science, 2004, 25(2):47-50(in Chinese)
王若师, 许秋瑾, 张娴, 等. 东江流域典型乡镇饮用水源地重金属污染健康风险评价[J]. 环境科学, 2012, 33(9):3083-3088Wang R S, Xu Q J, Zhang X, et al. Health risk assessment of heavy metals in typical township water sources in Dongjiang River Basin[J]. Environmental Science, 2012, 33(9):3083-3088(in Chinese)
张博文, 赵甲亭, 吴二威, 等. 滏阳河河流水体中重金属污染特征及其对青海弧菌和斜生栅藻的毒性效应[J]. 生态毒理学报, 2018, 13(1):179-189Zhang B W, Zhao J T, Wu E W, et al. Water pollution characteristics of heavy metals in Fuyang River system and their toxicity to Vibrio qinghaiensis sp. Q67 and Scenedesmus obliquus[J]. Asian Journal of Ecotoxicology, 2018, 13(1):179-189(in Chinese)
中华人民共和国卫生部, 中国国家标准管理委员会. 生活饮用水标准检验方法金属指标GB/T5750-2006[S]. 北京:中华人民共和国卫生部, 中国国家标准管理委员会, 2006
Wongsasuluk P, Chotpantarat S, Siriwong W, et al. Heavy metal contamination and human health risk assessment in drinking water from shallow groundwater wells in an agricultural area in Ubon Ratchathani Province, Thailand[J]. Environmental Geochemistry and Health, 2014, 36(1):169-182
United States Environmental Protection Agency (US EPA). Risk Assessment Guidance for Superfund. Volume 1. Human Health Evaluation Manual. Part A. (Interim Final). EPA/540/189/002; PB90-155581[R]. Washington DC:Office of Solid Waste and Emergency Response, US EPA, 1989
United States Environmental Protection Agency (US EPA). Guidance for performing aggregate exposure and risk assessments[R]. Washington DC:Office of Pesticide Programs, US EPA, 1999
United States Environmental Protection Agency (US EPA). Risk-based concentration table[R]. Washington DC:US EPA, 2000
World Health Organization (WHO). Trace elements in human nutrition and health[R]. Geneva:WHO, 1996
United States Environmental Protection Agency (US EPA). Guidelines for exposure assessment. EPA/600/Z-92/001.[R]. Washington DC:Risk Assessment Forum, US EPA, 1992
United States Environmental Protection Agency (US EPA). Guidelines for carcinogen risk assessment, NCEA-F-0644, review draft[R]. Washington DC:Risk Assessment Forum, US EPA, 1999
Cao H, Chen J, Zhang J, et al. Heavy metals in rice and garden vegetables and their potential health risks to inhabitants in the vicinity of an industrial zone in Jiangsu, China[J]. Journal of Environmental Sciences, 2010, 22(11):1792-1799
Zhu M, Jiang Y, Cui B, et al. Determination of the heavy metal levels in Panax Notoginseng and the implications for human health risk assessment[J]. Human & Ecological Risk Assessment, 2014, 21:1218-1229
Jiang Y, Zeng X, Fan X, et al. Levels of arsenic pollution in daily foodstuffs and soils and its associated human health risk in a town in Jiangsu Province, China[J]. Ecotoxicology and Environmental Safety, 2015, 122:198-204
宋成冉. 农村饮水安全面临的主要问题及对策[J]. 中国高新技术企业, 2015(12):95-96
樊新刚, 米文宝, 马振宁, 等. 宁夏石嘴山河滨工业园区表层土壤重金属污染的时空特征[J]. 环境科学, 2013, 34(5):1887-1894Fan X G, Mi W B, Ma Z N, et al. Spatial and temporal characteristics of heavy metal concentration of surface soil in Hebin Industrial Park in Shizuishan Northwest China[J]. Environmental Science, 2013, 34(5):1887-1894(in Chinese)
Zhang J, Huang W W, Martin J M. Trace metals distribution in Huanghe (Yellow River) estuarine sediments[J]. Estuarine, Coastal and Shelf Science, 1988, 26(5):499-516
Liu C, Xu J, Liu C, et al. Heavy metals in the surface sediments in Lanzhou Reach of Yellow River, China[J]. Bulletin of Environmental Contamination and Toxicology, 2009, 82(1):26-30
Ma X, Zuo H, Liu J, et al. Distribution, risk assessment, and statistical source identification of heavy metals in aqueous system from three adjacent regions of the Yellow River[J]. Environmental Science and Pollution Research, 2016, 23(9):8963-8975
沈雁峰, 孙殿军, 赵新华, 等. 中国饮水型地方性砷中毒病区和高砷区水砷筛查报告[J]. 中国地方病学杂志, 2005, 24(2):172-175Shen Y F, Sun D J, Zhao X H, et al. Screening report in areas of endemic arsenic and high content of arsenic in China[J]. Chinese Journal of Endemiology, 2005, 24(2):172-175(in Chinese)

相关话题/健康 宁夏 概率 污染 农村