1.
Introduction
In the present time, the influence of different types of radiation processing on semiconductors is being intensively analyzed[1–3]. One actual reason of the processing is doping of semiconductor materials to manufacture p–n junctions, transistors and other electronic devices in different technological ways. Another reason for analysis of influence of radiation processing on semiconductor materials is random impacts of radiation particles from cosmos irradiation or from other sources. Based on the analysis several recommendations to increase radiation resistance have been formulated[4–6]. One of them is choosing of materials with higher radiation resistance. Another one is using overlayers to decrease influence of undesirable irradiation. The third one is using annealing of radiation defects to decrease their quantity.
In this paper we analyze redistribution of point radiation defects, interaction between themselves and redistribution of their simplest complexes in multilayer structures. The analysis shows nonmonotonicity of distributions of concentrations of radiation defects, which recently was found experimentally[7]. To make the analysis we improve the model of analysis in comparison with previous references and used a recently introduced analytical approach to analyze these processes without crosslinking of solutions in layers of these structures.
2.
Method of solution
We determine spatio-temporal distributions of concentrations of point defects by solution of the following system of equations[8, 9].
$$begin{split}frac{{partial ,I,left( {r,z,t} ight)}}{{partial ,t}}= ,,& frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,{D_I}left( {z,T} ight)frac{{partial ,I,left( {r,z,t} ight)}}{{partial ,r}}} ight] + frac{{partial ,}}{{partial ,z}}left[ {{D_I}left( {z,T} ight)frac{{partial ,I,left( {r,z,t} ight)}}{{partial ,z}}} ight] - {K_I}left( {z,T} ight),{I^2}left( {r,z,t} ight) & -{K_r}[left( {z,T} ight),I,left( {r,z,t} ight),V,left( {r,z,t} ight) - {K_{rs}}left( {z,T} ight),I,left( {r,z,t} ight),V,left( {r,z,t} ight),,exp ,,left[ { - {{left( {z - {z_1}} ight)}^2}/{sigma ^2}} ight],frac{{partial ,V,left( {r,z,t} ight)}}{{partial ,t}} =, ,& frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,{D_V}left( {z,T} ight)frac{{partial ,V,left( {r,z,t} ight)}}{{partial ,r}}} ight] + frac{{partial ,}}{{partial ,z}}left[ {{D_V}left( {z,T} ight)frac{{partial ,V,left( {r,z,t} ight)}}{{partial ,z}}} ight] - {K_V}left( {z,T} ight),{V^2}left( {r,z,t} ight)&- {K_r}left( {z,T} ight),I,left( {r,z,t} ight),V,left( {r,z,t} ight) - {K_{rs}}left( {z,T} ight),I,left( {r,z,t} ight),V,left( {r,z,t} ight),,exp ,,left[ { - {{left( {z - {z_1}} ight)}^2}/{sigma ^2}} ight].end{split}$$ ![]() | (1) |
Here I (r, z, t) and V (r, z, t) are the spatio-temporal distributions of concentrations of interstitials and vacancies. The first terms of these equations describe diffusion of radiation defects. One can find dependence of diffusion coefficients Dρ (in diffusion terms of Eq. (1)) of defects on coordinate z due to presence of several layers framework of the considered multilayer structure. The second and the third terms of Eq. (1) describe generation of the simplest complexes of radiation defects and recombination of point radiation defects, respectively. The Eq. (1) should be complemented by boundary and initial conditions. We consider such boundary and initial conditions, which corresponds to absence of flow of defects through external boundary of the considered multilayer structure and distributions of concentrations of defects before starting of their stabilization. These conditions could be written as:
$$begin{split}& {left. {rfrac{{partial ,I,left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = 0}} = 0,;{left. {rfrac{{partial ,V,left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = 0}} = 0,;{left. {rfrac{{partial ,I,left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = R}} = 0,;{left. {rfrac{{partial ,V,left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = R}} = 0,{left. {frac{{partial ,I,left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = 0}} = 0,;{left. {frac{{partial ,V,left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = 0}} = 0, !! &;{left. {frac{{partial ,I,left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = L}} = 0,;{left. {frac{{partial ,V,left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = L}} = 0, ,, I,left( {r,z,0} ight) = {N_I}exp ,left[ { - frac{{{{left( {z - {z_{0I}}} ight)}^2}}}{{z_{I}^2}}} ight],;V,left( {r,z,0} ight) = {N_V}exp ,left[ { - frac{{{{left( {z - {z_{ m {0V}}}} ight)}^2}}}{{z_{V}^2}}} ight].end{split}$$ ![]() | (2) |
To simplify solution of Eq. (1) we transform these differential equations to the following integral form:
$$begin{split}& I,left( {r,z,t} ight) = frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_I}left( {z,T} ight)frac{{partial ,I,left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{{partial ,}}{{partial ,z}}left[ {intlimits_0^t {{D_{I}}left( {z,T} ight)frac{{partial ,I,left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] + I,left( {r,z,0} ight) [-4pt]& qquad - intlimits_0^t {{K_{r}}left( {z,T} ight),I,left( {r,z,tau } ight),V,left( {r,z,tau } ight),{ m d},tau } + intlimits_0^t {{K_{rs}}left( {z,T} ight),I,left( {r,z,tau } ight),,V,left( {r,z,tau } ight),,{ m d},tau } ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight] - intlimits_0^t {{K_{I}}left( {z,T} ight),{I^2}left( {r,z,tau } ight),{ m d},tau }, [-4pt]& V,left( {r,z,t} ight) = frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{V}}left( {z,T} ight)frac{{partial ,V,left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{{partial ,}}{{partial ,z}}left[ {intlimits_0^t {{D_{V}}left( {z,T} ight)frac{{partial ,V,left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] + V,left( {r,z,0} ight) [-4pt] & qquad - intlimits_0^t {{K_{r}}left( {z,T} ight),I,left( {r,z,tau } ight),V,left( {r,z,tau } ight),{ m d},tau } + intlimits_0^t {{K_{{rs}}}left( {z,T} ight),I,left( {r,z,tau } ight),,V,left( {r,z,tau } ight),,{ m d},tau } ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight] - intlimits_0^t {{K_{V}}left( {z,T} ight),{V^2}left( {r,z,tau } ight),{ m d},tau } .,,,,,,(1{ m a})end{split}$$ ![]() |
Now we will solve Eq. (1a) by method of averaging of function corrections[10] with decreasing quantity of iteration steps[11]. For the framework of the approach we used solutions of linear Eq. (1) with averaged diffusion coefficients D0IV as initial-order approximations of solutions of Eq. (1a). These initial-order approximations could be solved by standard Fourier approach[12, 13] and could be written as:
$$begin{split}&{I_0}left( {r,z,t} ight) = {F_{0I}} + sumlimits_{n = 1}^infty {{F_{nI}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0I}}t}}{{{L^2}}}} ight)} ,&{V_0}left( {r,z,t} ight) = {F_{0V}} + sumlimits_{n = 1}^infty {{F_{nV}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0V}}t}}{{{L^2}}}} ight)} .end{split}$$ ![]() |
Here
ight)int_0^L {I,left( {u,v,0}
ight),,cos ,left( {frac{{pi ,n,v}}{L}}
ight){text{d}}v{text{d}}u} ,}$
![](http://www.jos.ac.cn/article/id/17080024_M1.png)
ight)} int_0^L {V,left( {u,v,0}
ight)} ,,cos ,left( {frac{{pi ,n,v}}{L}}
ight){text{d}}v{text{d}}u$
![](http://www.jos.ac.cn/article/id/17080024_M2.png)
$$begin{split}{I_1}left( {r,z,t} ight) = ,, &frac{R}{{{r^2}}}sumlimits_{n = 1}^infty {{F_{nI}},cos ,left( {frac{{pi ,n,z}}{L}} ight),,left[ {intlimits_0^t {{D_I}left( {z,T} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0I}}t}}{{{L^2}}}} ight),{ m d},tau } + rintlimits_0^t {exp ,left( { - frac{{{pi ^2}{n^2}{D_{0I}}t}}{{{L^2}}}} ight)} ,, times ,, frac{{partial {D_I}left( {z,T} ight)}}{{partial r}} { m d} tau } ight.} [-1pt]&left. { - ,, R intlimits_0^t {{D_I}left( {z,T} ight) exp left( { - frac{{{pi ^2}{n^2}{D_{0I}}t}}{{{L^2}}}} ight) { m d} tau } } ight] {J_1}left( {nfrac{r}{R}} ight) - frac{pi }{L}sumlimits_{n = 1}^infty {n {F_{nI}} Bigggr[{20} {sin left( {frac{{pi n z}}{L}} ight) times intlimits_0^t {frac{{partial {D_I}left( {z,T} ight)}}{{partial z}} exp left( { - frac{{{pi ^2}{n^2}{D_{0I}}t}}{{{L^2}}}} ight) { m d} tau } }} [-1pt]& left. { + ,,frac{{pi n}}{L}cos left( {frac{{pi n z}}{L}} ight)intlimits_0^t {frac{{partial {D_I}left( {z,T} ight)}}{{partial z}} exp left( { - frac{{{pi ^2}{n^2}{D_{0I}}t}}{{{L^2}}}} ight) { m d} tau } } ight] times {J_0}left( {nfrac{r}{R}} ight),, - intlimits_0^t {{K_r}left( {z,T} ight)} [-2pt]& times ,,left[ {sumlimits_{n = 1}^infty {{F_{nI}}{J_0}left( {nfrac{r}{R}} ight) cos left( {frac{{pi n z}}{L}} ight) exp left( { - frac{{{pi ^2}{n^2}{D_{0I}}tau }}{{{L^2}}}} ight)} + frac{{{F_{0I}}}}{2}} ight] left[ {sumlimits_{n = 1}^infty {{J_0}left( {nfrac{r}{R}} ight) ,,times ,, {F_{nV}} cos left( {frac{{pi n z}}{L}} ight) exp left( { - frac{{{pi ^2}{n^2}{D_{0V}}tau }}{{{L^2}}}} ight)} } ight.[-2pt] & { + frac{{{F_{0V}}}}{2}} Bigggr]{20} d tau - {intlimits_0^t {{K_I}left( {z,T} ight)left[ {frac{{{F_{0I}}}}{2} + sumlimits_{n = 1}^infty {{F_{nI}} cos left( {frac{{pi n z}}{L}} ight) ,,times,, {J_0}left( {nfrac{r}{R}} ight) exp left( { - frac{{{pi ^2}{n^2}{D_{0I}}tau }}{{{L^2}}}} ight)} } ight] } ^2}{ m d} tau [-2pt] & + intlimits_0^t {left[ {sumlimits_{n = 1}^infty {{F_{nI}}{J_0}left( {frac{r}{R}} ight) cos left( {frac{{pi n z}}{L}} ight) exp left( { - frac{{{pi ^2}{n^2}{D_{0I}}tau }}{{{L^2}}}} ight)} + {F_{0I}}} ight]{K_{rs}}left( {z,T} ight)} [-2pt] & times ,, left[ {{F_{0V}} + sumlimits_{n = 1}^infty {{F_{nV}}{J_0}left( {frac{r}{R}} ight) cos left( {frac{{pi n z}}{L}} ight) exp left( { - frac{{{pi ^2}{n^2}{D_{0V}}tau }}{{{L^2}}}} ight)} } ight] { m d} tau exp left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight] + I left( {r,z,0} ight),end{split}$$ ![]() |
$$begin{split}{V_1}left( {r,z,t} ight) = & frac{R}{{{r^2}}}sumlimits_{n = 1}^infty {{F_{nV}}, cos , left( {frac{{pi , n, z}}{L}} ight), , left[ {intlimits_0^t {{D_V}left( {z,T} ight), exp , left( { - frac{{{pi ^2}{n^2}{D_{0V}}t}}{{{L^2}}}} ight), {text{d}}, tau } + rintlimits_0^t {exp , left( { - frac{{{pi ^2}{n^2}{D_{0V}}t}}{{{L^2}}}} ight) ,, times , , frac{{partial , {D_{{V}}}left( {z,T} ight)}}{{partial , r}}, {text{d}}, tau } , , } ight.} &left. { - R, intlimits_0^t {{D_{{V}}}left( {z,T} ight), exp , left( { - frac{{{pi ^2}{n^2}{D_{{{0V}}}}t}}{{{L^2}}}} ight), {text{d}}, tau } } ight], {J_1}left( {nfrac{r}{R}} ight), , - frac{pi }{L}sumlimits_{n = 1}^infty {n, {F_{{{nV}}}}, Bigggr[{20} {sin , left( {frac{{pi , n, z}}{L}} ight), , }} times intlimits_0^t {frac{{partial , {D_{{V}}}left( {z,T} ight)}}{{partial , z}}, exp , left( { - frac{{{pi ^2}{n^2}{D_{{{0V}}}}t}}{{{L^2}}}} ight), , {text{d}}, tau } &left. { + frac{{pi , n}}{L}cos , left( {frac{{pi , n, z}}{L}} ight)intlimits_0^t {frac{{partial , {D_{{V}}}left( {z,T} ight)}}{{partial , z}}, exp , left( { - frac{{{pi ^2}{n^2}{D_{{{0V}}}}t}}{{{L^2}}}} ight), { m d}, tau } } ight] times ,{J_0}left( {nfrac{r}{R}} ight) & - intlimits_0^t {{K_{r}}left( {z,T} ight),,left[ {sumlimits_{n = 1}^infty {{F_{nI}}{J_0}left( {nfrac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{{0I}}}tau }}{{{L^2}}}} ight)} + frac{{{F_{{0I}}}}}{2}} ight],left[ {sumlimits_{n = 1}^infty {{J_0}left( {nfrac{r}{R}} ight),, } } ight.} & { times ,,{F_{nV}},cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0V}}tau }}{{{L^2}}}} ight) + frac{{{F_{0V}}}}{2}} Bigggr]{20} ,,{ m d},tau - intlimits_0^t {{K_{V}}left( {z,T} ight),left[ {frac{{{F_{0V}}}}{2} + sumlimits_{n = 1}^infty {{F_{{nV}}},cos ,left( {frac{{pi ,n,z}}{L}} ight) } } ight.} & {left. { times ,,{J_0}left( {nfrac{r}{R}} ight),,exp ,left( { - frac{{{pi ^2}{n^2}{D_{0V}}tau }}{{{L^2}}}} ight)} ight]^2}{ m d},tau + intlimits_0^t {,left[ {sumlimits_{n = 1}^infty {{F_{nI}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0I}}tau }}{{{L^2}}}} ight)} } ight.} { +,, {F_{0I}}} Bigggr]{20}× {K_{rs}}left( {z,T} ight),left[ {{F_{{0V}}} + sumlimits_{n = 1}^infty {{F_{{nV}}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{{0V}}}tau }}{{{L^2}}}} ight)} } ight],,{ m d},tau ,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight] &+ V,left( {r,z,0} ight).end{split}$$ ![]() |
We determine the second- and highest-orders of approximations of concentrations of point radiation defects framework standard iterative procedure of method of averaging of function corrections[10]. In this case n-th-order approximations of concentrations of defects will be determined by following replacement I (r, z, t)→αnI + In?1 (r, z, t), V (r, z, t)→αnV + Vn?1 (r, z, t) in right sides of Eq. (1a), where αnI and αnV are the average values of the considered approximations. In this situation the second-order approximations of concentrations of point defects could be written as:
$$begin{split}{I_2}left( {r,z,t} ight) = ,, &frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{I}}left( {z,T} ight)frac{{partial ,{I_1}left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{{partial ,}}{{partial ,z}}left[ {intlimits_0^t {{D_{ I}}left( {z,T} ight)frac{{partial ,{I_1}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] [-2pt]& - intlimits_0^t {{K_{r}}left( {z,T} ight),left[ {{alpha _{{2I}}} + {I_1}left( {r,z,tau } ight)} ight],left[ {{alpha _{2V}} + {V_1}left( {r,z,tau } ight)} ight],,{ m d},tau } - intlimits_0^t {{K_I}left( {z,T} ight),{{left[ {{alpha _{2I}} + {I_1}left( {r,z,tau } ight)} ight]}^2},{ m d},tau } [-2pt]&- intlimits_0^t {{K_{{rs}}}left( {z,T} ight),left[ {{alpha _{2I}} + {I_1}left( {r,z,tau } ight)} ight],left[ {{alpha _{2V}} + {V_1}left( {r,z,tau } ight)} ight],,{ m d},tau ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight]} + I,left( {r,z,0} ight),[-1pt]{V_2}left( {r,z,t} ight) =,,& frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{V}}left( {z,T} ight)frac{{partial ,{V_1}left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{{partial ,}}{{partial ,z}}left[ {intlimits_0^t {{D_{V}}left( {z,T} ight)frac{{partial ,{V_1}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] [-1pt]& - intlimits_0^t {{K_{r}}left( {z,T} ight),left[ {{alpha _{{2I}}} + {I_1}left( {r,z,tau } ight)} ight],left[ {{alpha _{{2V}}} + {V_1}left( {r,z,tau } ight)} ight],,{ m d},tau } - intlimits_0^t {{K_{V}}left( {z,T} ight),{{left[ {{alpha _{{2V}}} + {V_1}left( {r,z,tau } ight)} ight]}^2},{ m d},tau }[-1pt] & - intlimits_0^t {{K_{rs}}left( {z,T} ight),left[ {{alpha _{ {2I}}} + {I_1}left( {r,z,tau } ight)} ight],left[ {{alpha _{{2V}}} + {V_1}left( {r,z,tau } ight)} ight],,{ m d},tau ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight]} + V,left( {r,z,0} ight).end{split}$$ ![]() |
Average values of the second-order approximations of the considered concentrations could be determined by the following standard relations
$${alpha _{2I}} = frac{2}{{Theta {R^2}L}}intlimits_0^Theta {intlimits_0^R {rintlimits_0^L {left[ {{I_2}left( {r,z,t} ight) - {I_1}left( {r,z,t} ight)} ight]{{ m d}z{ m d}r{ m d}t}} } } , quad {alpha _{2V}} = frac{2}{{Theta {R^2}L}}intlimits_0^Theta {intlimits_0^R {rintlimits_0^L {left[ {{V_2}left( {r,z,t} ight) - {V_1}left( {r,z,t} ight)} ight]{{ m d}z{ m d}r{ m d}t}} } } .$$ ![]() |
Substitution of the appropriate approximations of concentrations of point defects into above relations leads to the following relations
$$begin{split}& {alpha _{2I}} = frac{1}{{2{A_{II00}}}}{left{ {{{left( {1 + {A_{IV01}} + {A_{II10}} + {alpha _{2V}}{A_{IV00}}} ight)}^2} - 4{A_{II00}}left[ {{alpha _{2V}}{A_{IV10}} - {A_{II20}} + {A_{IV11}}{kern 1pt} {kern 1pt} - left. {frac{2}{{{R^2}L}}intlimits_0^R {rintlimits_0^L {I{kern 1pt} left( {r,z,0} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} r} } } ight]} ight.} ight}^{frac{1}{2}}}[-3pt] & qquad - frac{{1 + {A_{IV01}} + {A_{II10}} + {alpha _{2V}}{A_{IV00}}}}{{2{kern 1pt} {A_{II00}}}},& {alpha _{2V}} = frac{1}{{2{B_4}}}sqrt {frac{{{{left( {{B_3} + A} ight)}^2}}}{4} - 4{B_4}left( {y + frac{{{B_3}y - {B_1}}}{A}} ight)} - frac{{{B_3} + A}}{{4{B_4}}},end{split}$$ ![]() |
where
$$begin{split}&{A_{{abij}}} = frac{2}{{Theta ,{R^2}L}}intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {rintlimits_0^L {{k_{a,b}}left( {z,T} ight),I_1^ileft( {r,z,t} ight),V_1^jleft( {r,z,t} ight){{ m d}z{ m d}r{ m d}t}} } },[-3pt] & {B_4} = A_{IV00}^2A_{IV00}^2 - 2,{left( {A_{IV00}^2 - {A_{II00}}{A_{VV00}}} ight)^2},[-3pt] & {B_3} = {A_{{{IV00}}}}A_{{{IV00}}}^2 ,,+,, {A_{{{IV01}}}}A_{{{IV00}}}^3{ m{ ,,+,, }}{A_{{{IV00}}}}{A_{{{II10}}}}A_{{{IV00}}}^2 ,-,, 4 {A_{{{IV10}}}}{A_{{{II00}}}}A_{{{IV00}}}^2 ,,+,, 2 {A_{{{IV00}}}}{A_{{{IV01}}}}A_{{{IV00}}}^2 [-3pt] & quadquad - 4left[ {2{A_{{IV01}}}{A_{{IV00}}} + 2{A_{{IV00}}}} {left( {1 + {A_{{{IV01}}}} + {A_{{{II10}}}}} ight) - 2{A_{{{II00}}}}left( {{A_{{{IV10}}}} + {A_{{{VV10}}}} + 1} ight)} ight]left( {A_{{{IV00}}}^2 - {A_{{{II00}}}}{A_{{{VV00}}}}} ight),[-5pt] & {B_2} = A_{IV00}^2left{ {{kern 1pt} {{left( {1 + {A_{IV01}} + {A_{II10}}} ight)}^2} - {kern 1pt} left[ {{A_{IV11}} - {A_{II20}} - frac{1}{{{L_x}{L_y}{L_z}}}intlimits_0^{{L_x}} {intlimits_0^{{L_y}} {intlimits_0^{{L_z}} {{f_I}left( {x,y,z} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} y{kern 1pt} { m d}{kern 1pt} x} } } } ight]{kern 1pt} {kern 1pt} } ight.[-7pt]& quadquad { times {kern 1pt} {kern 1pt} 4{A_{II00}} + A_{IV00}^2A_{IV01}^2 + 2{kern 1pt} {A_{IV00}}{A_{IV01}}left( {{A_{IV00}} + {A_{IV00}}{A_{IV01}} + {A_{IV00}}{A_{II10}} - 4{A_{IV10}}{A_{II00}}} ight)} Bigggr}{22} {kern 1pt} left{ {left[ {2{A_{IV01}}{A_{IV00}}} ight.} ight.[-5pt]& quadquad {left. { + ,, 2{A_{IV00}}left( {1 + {A_{IV01}} + {A_{II10}}} ight) - 2{A_{II00}}left( {{A_{IV10}} + {A_{VV10}} + 1} ight)} ight]^2} + 2{kern 1pt} Bigggr[{20} {{A_{IV01}}left( {1 + {A_{IV01}} + {A_{II10}}} ight) + {A_{VV10}} + 1} [-5pt]& quadquad {left. { { +,, frac{4}{{{R^2}L}}intlimits_0^R {rintlimits_0^L {Vleft( {r,z,0} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} r} } - 2{A_{II00}}left( {{A_{VV20}} - {A_{IV11}}} ight)}} ight]^2} + 2{kern 1pt} left[ {frac{4}{{{R^2}L}}intlimits_0^R {rintlimits_0^L {Vleft( {r,z,0} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} r} } + {A_{IV01}}} ight.[-5pt] & quadquad { times {kern 1pt} {kern 1pt} left( {{A_{IV01}} + {A_{II10}} + 1} ight) - 2{A_{II00}}left( {{A_{VV20}} - {A_{IV11}}} ight) + {A_{IV01}}left( {1 + {A_{IV01}} + {A_{II10}}} ight)} Bigggr]{20} {kern 1pt} left[ {2{A_{IV00}}left( {1 + {A_{IV01}} + {A_{II10}}} ight)} ight.[-3pt]& quadquad left. {left. { - ,, 2{A_{II00}}left( {{A_{IV10}} + {A_{VV10}} + 1} ight) + 2{A_{IV01}}{A_{IV00}}} ight]} ight},[-4pt] & {B_1} = 2{A_{IV00}}{A_{IV01}}{left( {1 + {A_{IV01}} + {A_{II10}}} ight)^2} -,, 8{kern 1pt} {A_{IV00}}{A_{IV01}}{A_{II00}}[-5pt] & qquad times left[ {{A_{IV11}} - ,,{A_{II20}} - frac{2}{{{R^2}L}}intlimits_0^R {rintlimits_0^L {intlimits_0^{{L_z}} {I{kern 1pt} left( {r,z,0} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} r} } } } ight]{kern 1pt} + A_{IV01}^2 ( {{A_{IV00}} + {A_{IV00}}{A_{IV01}} - ,,4{A_{IV10}}{A_{II00}}}+{{A_{IV00}}{A_{II10}}} )[-4pt] & qquad - ,, 2{kern 1pt} left[ {frac{{4{A_{II00}}}}{{{R^2}L}}intlimits_0^R {rintlimits_0^L {I{kern 1pt} left( {r,z,0} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} r} } + {A_{IV01}}left( {1 + {A_{IV01}} + {A_{II10}}} ight) + {A_{IV01}}left( {1 + {A_{IV01}} + {A_{II10}}} ight)} ight.[-4pt] & qquad { -,, 2{A_{II00}}left( {{A_{VV20}} - {A_{IV11}}} ight)} Bigggr]{22}{kern 1pt} left[ {2{A_{IV00}}left( {1 + {A_{IV01}} + {A_{II10}}} ight) - 2{kern 1pt} {A_{II00}}left( {{A_{IV10}} + {A_{VV10}} + 1} ight) + 2{A_{IV01}}{A_{IV00}}} ight],[-4pt] & {{B_0} = 4{A_{II00}}A_{IV01}^2left[ {{A_{II20}} + frac{4}{{{R^2}L}}intlimits_0^R {rintlimits_0^L {I{kern 1pt} left( {r,z,0} ight){kern 1pt} { m d}{kern 1pt} z{kern 1pt} { m d}{kern 1pt} r} } - {A_{IV11}}} ight] + A_{IV01}^2{{left( {{A_{IV01}} + {A_{II10}} + 1} ight)}^2} - Bigggr[{22} {frac{{4{A_{II00}}}}{{{R^2}L}} }}[-4pt]& qquad {{{left. { times intlimits_0^R {rintlimits_0^L {V{kern 1pt} left( {r,z,0} ight){kern 1pt} d{kern 1pt} z{kern 1pt} d{kern 1pt} r} } + {A_{IV01}}left( {1 + {A_{IV01}} + {A_{II10}}} ight) - 2{A_{II00}}left( {{A_{VV20}} - {A_{IV11}}} ight) + {A_{IV01}}left( {1 + {A_{IV01}} + {A_{II10}}} ight)} ight]}^2}},[-3pt] & y = frac{{{B_2}}}{6} + sqrt[3]{{sqrt {{q^2} + {p^3}} - q}} - sqrt[3]{{sqrt {{q^2} + {p^3}} + q}},quad A = sqrt {8y + B_3^2 - 4{B_2}},[-3pt] & q = left( {2{B_1}{B_3} - 8{B_0}} ight)frac{{{B_2}}}{{48}} + frac{{B_2^3}}{{216}} + frac{{{B_0}left( {4{B_2} - B_3^2} ight) - B_1^2}}{8},quad {kern 1pt} p = frac{{{B_1}{B_3}}}{{12}} - frac{{{B_0}}}{3} - frac{{B_2^2}}{{36}}.end{split}$$ ![]() |
Θ is the continuance of observation of variation in time of the concentrations of these defects. Equations for concentrations of simplest complexes of point defects (divacancies ΦV(r, z, t) and diinterstitials ΦI(r, z, t)) could be written as
$$begin{split}frac{{partial ,,{varPhi _I}left( {r,z,t} ight)}}{{partial ,,t}} = &frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,{D_I}left( {z,T} ight)frac{{partial ,I,left( {r,z,t} ight)}}{{partial ,r}}} ight] + frac{partial }{{partial ,,z}}left[ {{D_{varPhi I}}left( {z,T} ight)frac{{partial ,{varPhi _I}left( {r,z,t} ight)}}{{partial ,z}}} ight] & + ,, {k_{I,I}}left( {z,T} ight),{I^2}left( {r,z,t} ight) - {k_I}left( {z,T} ight),I,left( {r,z,t} ight) + {K_{rs}}left( {z,T} ight),{varPhi _I}left( {r,z,t} ight),{varPhi _V},left( {r,z,t} ight),,exp ,,left[ { - {{left( {z - {z_1}} ight)}^2}/{sigma ^2}} ight],frac{{partial ,,{varPhi _V}left( {x,y,z,t} ight)}}{{partial ,,t}} = & frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,{D_V}left( {z,T} ight)frac{{partial ,V,left( {r,z,t} ight)}}{{partial ,r}}} ight] + frac{partial }{{partial ,,z}}left[ {{D_{varPhi V}}left( {z,T} ight)frac{{partial ,{varPhi _V}left( {r,z,t} ight)}}{{partial ,z}}} ight] & + ,, {k_{V,V}}left( {z,T} ight),{V^2}left( {r,z,t} ight) - {k_V}left( {z,T} ight),V,left( {r,z,t} ight) + {K_{rs}}left( {z,T} ight),{varPhi _I}left( {r,z,t} ight),{varPhi _V},left( {r,z,t} ight),,exp ,,left[ { - {{left( {z - {z_1}} ight)}^2}/{sigma ^2}} ight],end{split}$$ ![]() | (3) |
with boundary and initial conditions
$$begin{split}& r{left. {frac{{partial ,{varPhi _I}left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = 0}} = 0,;r{left. {frac{{partial ,{varPhi _V}left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = 0}} = 0,;r{left. {frac{{partial ,{varPhi _I}left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = R}} = 0,;r{left. {frac{{partial ,{varPhi _V}left( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = R}} = 0,& {left. {frac{{partial ,{varPhi _I}left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = 0}} = 0,;{left. {frac{{partial ,{varPhi _V}left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = 0}} = 0,;{left. {frac{{partial ,{varPhi _I}left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = L}} = 0,;{left. {frac{{partial ,{varPhi _V}left( {r,z,t} ight)}}{{partial ,z}}} ight|_{z = L}} = 0,& {varPhi _I}left( {r,z,0} ight) = {N_{{varPhi _I}}}exp ,left[ { - frac{{{{left( {z - {z_{0{varPhi _I}}}} ight)}^2}}}{{z_{{varPhi _I}}^2}}} ight],;{varPhi _V}left( {r,z,0} ight) = {N_{{varPhi _V}}}exp ,left[ { - frac{{{{left( {z - {z_{0{varPhi _V}}}} ight)}^2}}}{{z_{{varPhi _V}}^2}}} ight].end{split}$$ ![]() | (4) |
Here DΦρ(z, T) are the diffusion coefficients of the above complexes of radiation defects; kρ(z, T) are the parameters of decay of the above complexes. To simplify solution of the above equations we transform them to the following integral form
$$begin{split}quadqquad{varPhi _I}left( {r,z,t} ight)= ,, & frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight)frac{{partial ,{varPhi _I}left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{partial }{{partial ,,z}}left[ {intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight)frac{{partial ,{varPhi _I}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] & + intlimits_0^t {{k_{I,I}}left( {z,T} ight),{I^2}left( {r,z,tau } ight),{ m d},tau } - intlimits_0^t {{k_I}left( {z,T} ight),I,left( {r,z,tau } ight),{ m d},tau } + intlimits_0^t {{K_{rs}}left( {z,T} ight),{varPhi _I}left( {r,z,tau } ight),{varPhi _V},left( {r,z,tau } ight),{ m d},tau } & times ,,exp ,,left[ { - {{left( {z - {z_1}} ight)}^2}/{sigma ^2}} ight] + {varPhi _I}left( {r,z,0} ight),{varPhi _V}left( {r,z,t} ight) = & frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight)frac{{partial ,{varPhi _I},left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{partial }{{partial ,,z}}left[ {intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight)frac{{partial ,{varPhi _V}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] & + intlimits_0^t {{k_{V,V}}left( {z,T} ight),{V^2}left( {r,z,tau } ight),{ m d},tau } - intlimits_0^t {{k_V}left( {z,T} ight),V,left( {r,z,tau } ight),{ m d},tau } + intlimits_0^t {{K_{rs}}left( {z,T} ight),{varPhi _I}left( {r,z,tau } ight),{varPhi _V},left( {r,z,tau } ight),{ m d},tau } & times ,,exp ,,left[ { - {{left( {z - {z_1}} ight)}^2}/{sigma ^2}} ight] + {varPhi _V}left( {r,z,0} ight).qquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquadquad(3{ m a})end{split}$$ ![]() |
Now we solve systems of Eq. (3a) by method of averaging of function corrections with decreasing quantity of iteration steps. For the framework of the approach we used solutions of Eq. (3) with averaged diffusion coefficients D0IV and without any nonlinearity on concentration of defects as initial-order approximations of solutions of Eq. (3a). These initial-order approximations could be solved by standard Fourier approach and could be written as
$$begin{split}{varPhi _{I0}}left( {r,z,t} ight) = {F_{0{varPhi _I}}} + sumlimits_{n = 1}^infty {{F_{n{varPhi _I}}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}t}}{{{L^2}}}} ight)} ,{varPhi _{V0}}left( {r,z,t} ight) = {F_{0{varPhi _V}}} + sumlimits_{n = 1}^infty {{F_{n{varPhi _V}}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _V}}}t}}{{{L^2}}}} ight)} .end{split}$$ ![]() |
Here
ight){kern 1pt} } int_0^L {{varPhi _I}left( {u,v,0}
ight){kern 1pt} {kern 1pt} cos {kern 1pt} left( {frac{{pi {kern 1pt} n{kern 1pt} v}}{L}}
ight){kern 1pt} {text{d}}v{text{d}}u} $
![](http://www.jos.ac.cn/article/id/17080024_M13.png)
ight)} int_0^L {{varPhi _V},left( {u,v,0}
ight),cos ,left( {frac{{pi ,n,v}}{L}}
ight){text{d}}v{text{d}}u} $
![](http://www.jos.ac.cn/article/id/17080024_M14.png)
$$begin{split} {varPhi _{I1}}left( {r,z,t} ight) =,, & frac{R}{{{r^2}}}sumlimits_{n = 1}^infty {{F_{n{varPhi _I}}}cos ,left( {frac{{pi ,n,z}}{L}} ight),left[ {r,intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight),{J_0}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight),{ m d},tau } } ight]} - frac{1}{r}sumlimits_{n = 1}^infty {{F_{n{varPhi _I}}} } & times ,,cos ,left( {frac{{pi ,n,z}}{L}} ight)intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight),{J_1}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight),{ m d},tau } - sumlimits_{n = 1}^infty {{F_{n{varPhi _I}}}cos ,left( {frac{{pi ,n,z}}{L}} ight)intlimits_0^t {frac{{partial ,{D_{{varPhi _I}}}left( {z,T} ight)}}{{partial ,r}},, } } & times ,{J_1}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight),,{ m d},tau - frac{{{pi ^2}}}{{{L^2}}}sumlimits_{n = 1}^infty {{n^2}{F_{n{varPhi _I}}}{J_0}left( {frac{r}{R}} ight)intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight)exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight),{ m d},tau } } & times ,,cos ,left( {frac{{pi ,n,z}}{L}} ight) ,,+ ,, {varPhi _I}left( {r,z,0} ight) - frac{pi }{L}sumlimits_{n = 1}^infty {n,{J_0}left( {frac{r}{R}} ight),,sin ,left( {frac{{pi ,n,z}}{L}} ight),intlimits_0^t {frac{{partial ,{D_{{varPhi _I}}}left( {z,T} ight)}}{{partial ,,z}}exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight),{ m d},tau } ,, } & times {F_{n{varPhi _I}}} ,,+ ,,intlimits_0^t {{k_{I,I}}left( {z,T} ight),{I^2}left( {r,z,tau } ight),{ m d},tau } - intlimits_0^t {{k_I}left( {z,T} ight),I,left( {r,z,tau } ight),{ m d},tau } + intlimits_0^t {{K_{rs}}left( {z,T} ight),left[ {sumlimits_{n = 1}^infty {{F_{n{varPhi _I}}},cos ,left( {frac{{pi ,n,z}}{L}} ight) } } ight.} & left. { times ,, {J_0}left( {frac{r}{R}} ight),,exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight) + {F_{0{varPhi _I}}}} ight],left[ {sumlimits_{n = 1}^infty {{F_{n{varPhi _V}}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight)} } ight. & { + ,,{F_{0{varPhi _V}}}} Bigggr]{20} ,,{ m d},tau ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma^2}}}} ight],end{split}$$ ![]() |
$$begin{split} {varPhi _{V1}}left( {r,z,t} ight) = ,,&frac{R}{{{r^2}}}sumlimits_{n = 1}^infty {{F_{n{varPhi _V}}}cos ,left( {frac{{pi ,n,z}}{L}} ight),left[ {r,intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight),{J_0}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _V}}}tau }}{{{L^2}}}} ight),{ m d},tau } } ight]} - frac{1}{r}sumlimits_{n = 1}^infty {{F_{n{varPhi _V}}} } & times ,,cos ,left( {frac{{pi ,n,z}}{L}} ight)intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight),{J_1}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _V}}}tau }}{{{L^2}}}} ight),{ m d},tau } - sumlimits_{n = 1}^infty {{F_{n{varPhi _V}}}cos ,left( {frac{{pi ,n,z}}{L}} ight)intlimits_0^t {frac{{partial ,{D_{{varPhi _V}}}left( {z,T} ight)}}{{partial ,r}},, } } & times ,{J_1}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _V}}}tau }}{{{L^2}}}} ight),,{ m d},tau - frac{{{pi ^2}}}{{{L^2}}}sumlimits_{n = 1}^infty {{n^2}{F_{n{varPhi _V}}}{J_0}left( {frac{r}{R}} ight)intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight)exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _V}}}tau }}{{{L^2}}}} ight),{ m d},tau } } & times ,,cos ,left( {frac{{pi ,n,z}}{L}} ight) + {varPhi _V}left( {r,z,0} ight) - frac{pi }{L}sumlimits_{n = 1}^infty {n,{J_0}left( {frac{r}{R}} ight),,sin ,left( {frac{{pi ,n,z}}{L}} ight),intlimits_0^t {frac{{partial ,{D_{{varPhi _V}}}left( {z,T} ight)}}{{partial ,,z}}exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _V}}}tau }}{{{L^2}}}} ight),{ m d},tau } ,, } & times ,, {F_{n{varPhi _V}}} + intlimits_0^t {{k_{V,V}}left( {z,T} ight),{V^2}left( {r,z,tau } ight),{ m d},tau } - intlimits_0^t {{k_V}left( {z,T} ight),V,left( {r,z,tau } ight),{ m d},tau } + intlimits_0^t {{K_{rs}}left( {z,T} ight),left[ {sumlimits_{n = 1}^infty {{F_{n{varPhi _I}}},cos ,left( {frac{{pi ,n,z}}{L}} ight),, } } ight.} & left. { times,, {J_0}left( {frac{r}{R}} ight),,exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight) + {F_{0{varPhi _I}}}} ight],left[ {sumlimits_{n = 1}^infty {{F_{n{varPhi _V}}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{D_{0{varPhi _I}}}tau }}{{{L^2}}}} ight)} } ight.& { + ,, {F_{0{varPhi _V}}}} Bigggr]{20},,{ m d},tau ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight].end{split}$$ ![]() |
We determine the second- and highest-orders of approximations of concentrations of simplest complexes of point radiation defects framework standard iterative procedure of method of averaging of function corrections[10]. In this case n-th-order approximations of concentrations of complexes of defects will be determined by following replacement ΦI(r, z, t)→αnΦI +ΦIn-1(r, z, t), ΦV(r, z, t)→αnΦV + ΦVn-1(r, z, t) in right sides of Eq. (3a), where αnI and αnV are the average values of the considered approximations. In this situation the second-order approximations of concentrations of complexes of point defects could be written as
$$begin{split} {varPhi _{I2}}left( {r,z,t} ight) =,, &frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight)frac{{partial ,{varPhi _{I1}}left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{partial }{{partial ,,z}}left[ {intlimits_0^t {{D_{{varPhi _I}}}left( {z,T} ight)frac{{partial ,{varPhi _{I1}}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] & + intlimits_0^t {{K_{rs}}left( {z,T} ight),left[ {{alpha _{2{varPhi _I}}} + {varPhi _{1I}}left( {r,z,tau } ight)} ight],,left[ {{alpha _{2{varPhi _V}}} + {varPhi _{1V}}left( {r,z,tau } ight)} ight],,{ m d},tau } ,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight] +,, {varPhi _I}left( {r,z,0} ight) & + intlimits_0^t {{k_{I,I}}left( {z,T} ight),{I^2}left( {r,z,tau } ight),{ m d},tau } ,, - intlimits_0^t {{k_I}left( {z,T} ight),I,left( {r,z,tau } ight),{ m d},tau } ,{varPhi _{V2}}left( {r,z,t} ight) = ,&, frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight)frac{{partial ,{varPhi _{I2}},left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } } ight] + frac{partial }{{partial ,,z}}left[ {intlimits_0^t {{D_{{varPhi _V}}}left( {z,T} ight)frac{{partial ,{varPhi _{V2}}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } } ight] & + intlimits_0^t {{K_{rs}}left( {z,T} ight),left[ {{alpha _{2{varPhi _I}}} + ,, {varPhi _{1I}}left( {r,z,tau } ight)} ight],,left[ {{alpha _{2{varPhi _V}}} + ,, {varPhi _{1V}}left( {r,z,tau } ight)} ight],,{ m d},tau } ,,exp ,,left[ { - frac{{{{left( {z - {z_1}} ight)}^2}}}{{{sigma ^2}}}} ight] +,, {varPhi _V}left( {r,z,0} ight) & + intlimits_0^t {{k_{V,V}}left( {z,T} ight),{V^2}left( {r,z,tau } ight),{ m d},tau } ,, - intlimits_0^t {{k_V}left( {z,T} ight),V,left( {r,z,tau } ight),{ m d},tau } .end{split}$$ ![]() |
We determine spatio-temporal distribution of temperature of local heating, generated during generation of radiation defects due to radiation processing, by solution of the following equation
$$cleft( T ight)frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,t}} = frac{1}{r}frac{{partial ,}}{{partial ,r}}left[ {r,lambda left( {z,T} ight)frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,r}}} ight] + frac{{partial ,}}{{partial ,z}}left[ {lambda left( {z,T} ight)frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,z}}} ight].$$ ![]() | (5) |
Temperature dependence of heat capacitance
![](http://www.jos.ac.cn/article/id/17080024_Z-20180408015309-1.png)
m{d}}}}
ight)}
ight]$
![](http://www.jos.ac.cn/article/id/17080024_M15.png)
ight){
m{ }} = {lambda _1}left( z
ight)left{ {1 + mu {{left[ {{T_{
m{d}}}/Tleft( {r,z,t}
ight)}
ight]}^varphi }}
ight}$
![](http://www.jos.ac.cn/article/id/17080024_M16.png)
$$begin{split}& {left. {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = 0}} = 0,;{left. {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = R}} = 0,; & {left. {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,z}}} ight|_{r = 0}} = 0,;{left. {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,r}}} ight|_{r = L}} = 0,;T(r,z,0) = {T_{ m r}}.end{split}$$ ![]() | (6) |
Here Tr is the room temperature. With account dependence of heat diffusion coefficient on temperature one can transform the Eq. (5) to the following differential (7a) or integral (7b) form
$$qquadbegin{split}frac{{{c_0}}}{{varPhi + 2}},frac{{partial ,{T^{varPhi + 2}}left( {r,z,t} ight)}}{{partial ,t}} = ,, & T,left( {r,z,t} ight)frac{{{lambda _1}left( z ight)}}{r}left[ {{T^varPhi }left( {r,z,t} ight) + mu ,T_{ m d}^varPhi } ight]frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,r}} - varPhi ,mu ,T_{ m d}^varPhi {lambda _1}left( z ight),Tleft( {r,z,t} ight),, & times,, {left[ {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,r}}} ight]^2} + {lambda _1}left( z ight),T,left( {r,z,t} ight),,left[ {{T^varPhi }left( {r,z,t} ight) + mu ,T_{ m d}^varPhi } ight],frac{{{partial ^2}T,left( {r,z,t} ight)}}{{partial ,{r^2}}} + ,left[ {{T^varPhi }left( {r,z,t} ight) + mu ,T_{ m d}^varPhi } ight]frac{{partial ,{lambda _1}left( z ight)}}{{partial ,z}}, & times ,,T,left( {r,z,t} ight),frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,z}} - varPhi ,mu ,T_{ m d}^varPhi {lambda _1}left( z ight),Tleft( {r,z,t} ight),,{left[ {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,z}}} ight]^2} + {lambda _1}left( z ight),T,left( {r,z,t} ight),frac{{{partial ^2}Tleft( {r,z,t} ight)}}{{partial ,{z^2}}} & times ,left[ {{T^varPhi }left( {r,z,t} ight) + mu ,T_{ m d}^varPhi } ight].qquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquadqquad!!!{ m {(7a)}}end{split}$$ ![]() |
$$qquadbegin{split}frac{{{T^{varPhi + 2}}left( {r,z,t} ight)}}{{varPhi + 2}} =& frac{{{lambda _1}left( z ight)}}{r}intlimits_0^t {T,left( {r,z,tau } ight),left[ {{T^varPhi }left( {r,z,tau } ight) + mu ,T_{ m d}^varPhi } ight]frac{{partial ,Tleft( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } - varPhi ,mu ,T_{ m d}^varPhi intlimits_0^t {,{{left[ {frac{{partial ,Tleft( {r,z,tau } ight)}}{{partial ,r}}} ight]}^2}} [-8pt] & times,, T,left( {r,z,tau } ight),{ m d},tau ,{lambda _1}left( z ight) + {lambda _1}left( z ight),intlimits_0^t {T,left( {r,z,tau } ight),,left[ {{T^varPhi }left( {r,z,tau } ight) + mu ,T_{ m d}^varPhi } ight],frac{{{partial ^2}T,left( {r,z,tau } ight)}}{{partial ,{r^2}}}{ m d},tau } + intlimits_0^t {T,left( {r,z,tau } ight)} ,, [-7pt] & times , frac{{partial ,Tleft( {r,z,tau } ight)}}{{partial ,z}}left[ {{T^varPhi }left( {r,z,tau } ight) + mu ,T_{ m d}^varPhi } ight],,{ m d},tau frac{{partial ,{lambda _1}left( z ight)}}{{partial ,z}} - varPhi ,mu ,T_{ m d}^varPhi {lambda _1}left( z ight),intlimits_0^t {T,left( {r,z,tau } ight),{{left[ {frac{{partial ,Tleft( {r,z,tau } ight)}}{{partial ,z}}} ight]}^2}{ m d},tau } [-7pt] & + {lambda _1}left( z ight),intlimits_0^t {,left[ {{T^varPhi }left( {r,z,tau } ight) + mu ,T_{ m d}^varPhi } ight]frac{{{partial ^2}Tleft( {r,z,tau } ight)}}{{partial ,{z^2}}}T,left( {r,z,tau } ight),{ m d},tau } + {T_{ m r}}.qquadqquadqquadqquadqquadquadqquadqquad{ m {(7b)}}end{split}$$ ![]() |
We solved the Eq. (7b) by method of averaging of function corrections with decreased quantity of iterative steps. For the framework of the approach we used solutions of Eq. (5) with averaged heat diffusion coefficients λ0 without any nonlinearity on temperature as initial-order approximations of solutions of Eq. (7b). These initial-order approximations could be solved by standard Fourier approach and could be written as
$${T_0}left( {r,z,t} ight) = frac{{{F_0}}}{2} + sumlimits_{n = 1}^infty {{F_n}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}t}}{{{L^2}{c_0}}}} ight)} .$$ ![]() |
Here
ight)int_0^L {Tleft( {u,v,0}
ight),cos ,left( {frac{{pi ,n,v}}{L}}
ight){text{d}}v{text{d}}u} } $
![](http://www.jos.ac.cn/article/id/17080024_M17.png)
$$begin{split} {c_0}frac{{T_1^{varPhi + 2}left( {r,z,t} ight)}}{{varPhi + 2}} = & - frac{{{lambda _1}left( z ight)}}{{r,R}}intlimits_0^t {left{ {{{left[ {frac{{{F_0}}}{2} + sumlimits_{m = 1}^infty {{F_m}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,m,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{m^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight},, } [-6pt] & times ,,left[ {frac{{{F_0}}}{2} + sumlimits_{l = 1}^infty {{F_l}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,l,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{l^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight],sumlimits_{n = 1}^infty {{F_n}{J_1}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} ,{ m d},tau [-6pt] & + ,, varPhi ,mu ,{lambda _1}left( z ight)frac{{T_{ m d}^varPhi }}{{{R^2}}}intlimits_0^t {{{left[ {sumlimits_{n = 1}^infty {{F_n}{J_1}left( {frac{r}{R}} ight)cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight]}^2}left[ {frac{{{F_0}}}{2} + sumlimits_{m = 1}^infty {{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,m,z}}{L}} ight),, } } ight.} [-6pt] & left. { times ,,{F_m}exp ,left( { - frac{{{pi ^2}{m^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} ight],{ m d},tau + {lambda _1}left( z ight),intlimits_0^t {left[ {frac{{{F_0}}}{2} + sumlimits_{m = 1}^infty {{F_m}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,m,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{m^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight],,left[ {frac{{{F_0}}}{2} } ight.} [-6pt] & {left. { + ,, {F_n}cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} ight]^2}{ m d},tau + {lambda _1}left( z ight),intlimits_0^t {left[ {sumlimits_{n = 1}^infty {{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} ,, } ight.} [-6pt] & left. { times ,, frac{{{F_n}}}{R} + frac{{{F_0}}}{2}} ight],left{ {{{left[ {frac{{{F_0}}}{2} + sumlimits_{m = 1}^infty {{F_m}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,m,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{m^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}sumlimits_{l = 1}^infty {{F_l}left[ {3frac{R}{r}{J_1}left( {frac{r}{R}} ight) } ight.,} [-6pt] & left. { + ,, {J_0}left( {frac{r}{R}} ight)} ight],cos ,left( {frac{{pi ,l,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{l^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight),{ m d},tau - frac{{partial ,{lambda _1}left( z ight)}}{{partial ,z}}intlimits_0^t {left[ {frac{{{F_0}}}{2} + sumlimits_{m = 1}^infty {{F_m}{J_0}left( {frac{r}{R}} ight),exp ,left( { - frac{{{pi ^2}{m^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight.} ,, [-6pt] & times ,, left. {cos ,left( {frac{{pi ,m,z}}{L}} ight)} ight]left{ {{{left[ {frac{{{F_0}}}{2} + sumlimits_{l = 1}^infty {{F_l}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,l,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{l^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}sumlimits_{n = 1}^infty {{F_n}frac{{pi ,n}}{L}{J_0}left( {frac{r}{R}} ight)} ,, [-6pt] & times ,,exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight),,{ m d},tau ,sin ,left( {frac{{pi ,n,z}}{L}} ight) - varPhi ,intlimits_0^t {{{left[ {sumlimits_{n = 1}^infty {frac{{pi ,n}}{L}{F_n}{J_0}left( {frac{r}{R}} ight),sin ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight]}^2}} [-6pt] & times ,, mu ,,T_{ m d}^varPhi {lambda _1}left( z ight)sumlimits_{l = 1}^infty {{F_l}{J_0}left( {frac{r}{R}} ight)cos ,left( {frac{{pi ,l,z}}{L}} ight)exp ,left( { - frac{{{pi ^2}{l^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight),{ m d},tau } - {pi ^2}{lambda _1}left( z ight),intlimits_0^t {left{ {left[ {frac{{{F_0}}}{2} + sumlimits_{m = 1}^infty {{F_m}{J_0}left( {frac{r}{R}} ight),,, } } ight.} ight.,} [-6pt] & left. { times ,,{{left. {cos ,left( {frac{{pi ,m,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{m^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}left[ {frac{{{F_0}}}{2} + sumlimits_{l = 1}^infty {{F_l}{J_0}left( {frac{r}{R}} ight),,cos ,left( {frac{{pi ,l,z}}{L}} ight)exp ,left( { - frac{{{pi ^2}{l^2}{lambda _0}tau }}{{{L^2}{c_0}}}} ight)} } ight],, [-6pt] & times ,,sumlimits_{n = 1}^infty {{F_n}frac{{{n^2}}}{{{L^2}}}{J_0}left( {frac{r}{R}} ight),cos ,left( {frac{{pi ,n,z}}{L}} ight),exp ,left( { - frac{{{pi ^2}{n^2}{lambda _0}t}}{{{L^2}{c_0}}}} ight)} ,{ m d},tau + {T_{ m r}}.end{split}$$ ![]() |
We determine the second- and highest-orders of approximation of temperature framework standard iterative procedure of method of averaging of function corrections[10]. In this case n-th-order approximation of temperature will be determined by following replacement T(r, z, t) → αnT + Tn-1(r, z, t) in right sides of Eq. (7b), where αnT is the average value of the considered approximation. In this situation the second-order approximation of temperature could be written as
$$begin{split}{c_0}frac{{T_2^{varPhi + 2}left( {r,z,t} ight)}}{{varPhi + 2}} =& frac{{{lambda _1}left( z ight)}}{r}intlimits_0^t {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],left{ {{{left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}frac{{partial ,{T_1}left( {r,z,tau } ight)}}{{partial ,r}}{ m d},tau } - varPhi ,mu ,, & times ,{lambda _1}left( z ight)T_{ m d}^varPhi intlimits_0^t {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],{{left[ {frac{{partial ,{T_1}left( {r,z,tau } ight)}}{{partial ,r}}} ight]}^2}{ m d},tau } + {lambda _1}left( z ight),intlimits_0^t {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],left{ {{{left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight]}^varPhi }} ight.} & left. { + ,, mu ,T_{ m d}^varPhi } ight},frac{{{partial ^2}{T_1}left( {r,z,tau } ight)}}{{partial ,{r^2}}}{ m d},tau ,, + intlimits_0^t {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],left{ {,{{left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}frac{{partial ,{T_1}left( {r,z,tau } ight)}}{{partial ,z}}{ m d},tau } ,, & times frac{{partial ,{lambda _1}left( z ight)}}{{partial ,z}} - varPhi ,mu ,T_{ m d}^varPhi {lambda _1}left( z ight),intlimits_0^t {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],{{left[ {frac{{partial ,Tleft( {r,z,tau } ight)}}{{partial ,z}}} ight]}^2}{ m d},tau } + {lambda _1}left( z ight),intlimits_0^t {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],} & times ,,left{ {,{{left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}frac{{{partial ^2}{T_1}left( {r,z,tau } ight)}}{{partial ,{z^2}}},{ m d},tau + {T_{ m r}}.end{split}$$ ![]() |
Not yet known average value α2T by solution of the following equation
$$begin{split}& frac{{{c_0}}}{{varPhi + 2}}intlimits_0^Theta {intlimits_0^R {rintlimits_0^L {T_2^{varPhi + 2}left( {r,z,t} ight),{ m d},z,{ m d},r,{ m d},t} } } = intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {intlimits_0^L {left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight],left{ {{{left[ {{alpha _{2T}} + {T_1}left( {r,z,tau } ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight},} } } & qquad times ,, {lambda _1}left( z ight)frac{{partial ,{T_1}left( {r,z,tau } ight)}}{{partial ,r}},{ m d},z,{ m d},r,{ m d},t - varPhi ,mu ,intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {intlimits_0^L {{lambda _1}left( z ight),left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight],{{left[ {frac{{partial ,{T_1}left( {r,z,t} ight)}}{{partial ,r}}} ight]}^2}{ m d},z,{ m d},r,{ m d},t} } } & qquad times,, T_{ m d}^varPhi + intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {intlimits_0^L {{lambda _1}left( z ight)left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight],left{ {{{left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight},frac{{{partial ^2}{T_1}left( {r,z,t} ight)}}{{partial ,{r^2}}}{ m d},z,{ m d},r,{ m d},t} } } & qquad + intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {intlimits_0^L {frac{{partial ,{lambda _1}left( z ight)}}{{partial ,z}}frac{{partial ,{T_1}left( {r,z,t} ight)}}{{partial ,z}}left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight],left{ {{{left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight},,{ m d},z,{ m d},r,{ m d},t} } } & qquad + intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {intlimits_0^L {{lambda _1}left( z ight)left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight],left{ {{{left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight]}^varPhi } + mu ,T_{ m d}^varPhi } ight}frac{{{partial ^2}{T_1}left( {r,z,t} ight)}}{{partial ,{z^2}}}{ m d},z,{ m d},r,{ m d},t} } } , & qquad - varPhi ,mu ,T_{ m d}^varPhi times intlimits_0^Theta {left( {Theta - t} ight)intlimits_0^R {intlimits_0^L {{lambda _1}left( z ight),left[ {{alpha _{2T}} + {T_1}left( {r,z,t} ight)} ight],{{left[ {frac{{partial ,Tleft( {r,z,t} ight)}}{{partial ,z}}} ight]}^2}{ m d},z,{ m d},r,{ m d},t} } } + Theta L{R^2}frac{{{T_{ m r}}}}{2}.end{split}$$ ![]() |
3.
Discussion
In this paper we analyzed spatio-temporal distributions of concentrations of radiation defects in a multilayer structure with account of spatio-temporal distribution of local heating, generated during generation of radiation defects due to radiation processing. Fig. 1 shows distribution of concentration of implanted dopant (curve 1), distribution of concentration of interstitials (curve 2) and distribution of concentration of vacancies (curve 3). In this figure, to the right of the maximum of the given concentrations, one can find a local minimum concentration of defects. The local minimum is presented on interface between layers of the considered multilayer structure. Recently the minimum has been experimentally obtained and discussed in Ref. [7]. Probably the interface between layers of multilayer structure could be considered as a drain of radiation defects. To take into account the drain we introduce last terms in Eq. (1).
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Figure1.
(Color online) Distribution of concentration for the implanted dopant (curve 1), interstitials (curve 2) and vacancies (curve 3). Solid lines are analytical results, and dashed lines are results from cluster dynamics model.
4.
Conclusion
In this paper we introduce a model of redistribution of point radiation defects, interaction between themselves and redistribution of their simplest complexes in multilayer structures. The model gives a possibility to qualitatively describe nonmonotonicity of distributions of concentrations of radiation defects, which recently was found experimentally. To take into account the nonmonotonicity we complement the model for analysis of distribution of concentration of radiation defects, which recently was used in literature. To analyze the model we used an approach of solution of boundary problems, which could be used without crosslinking of solutions on interfaces between layers of the considered multilayer structures.