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鄂尔多斯市夏秋季气溶胶新粒子生成过程影响因素分析

本站小编 Free考研考试/2021-12-31

中文关键词鄂尔多斯新粒子生成(NPF)气象要素气团类型粒径分布 英文关键词Ordosnew particle formation(NPF)meteorological elementair masssize distribution
作者单位E-mail
孔祥晨鄂尔多斯市气象局, 鄂尔多斯 017000
南京信息工程大学气象灾害预报预警与评估协同创新中心, 中国气象局气溶胶-云-降水重点开放实验室, 南京 210044
15147736650m@sina.cn
王红磊南京信息工程大学气象灾害预报预警与评估协同创新中心, 中国气象局气溶胶-云-降水重点开放实验室, 南京 210044hongleiwang@nuist.edu.cn
张连霞鄂尔多斯市气象局, 鄂尔多斯 017000
呼群鄂尔多斯市气象局, 鄂尔多斯 017000
李瑞锋鄂尔多斯市气象局, 鄂尔多斯 017000
许彩琴鄂尔多斯市气象局, 鄂尔多斯 017000
中文摘要 利用宽范围粒径谱仪于2019年8月16至10月4日在鄂尔多斯市观测了10 nm~10 μm气溶胶粒径分布,结合PM(PM2.5和PM10)、污染气体、气象数据和HYSPLIT模式,分析了新粒子生成(NPF)特征及其主要影响因素.结果表明,观测期间一共出现19次NPF过程,占总观测期间的37.5%.NPF过程中对不同模态气溶胶数浓度日变化的影响不同.NPF使得核模态和爱根核模态气溶胶数浓度急剧增加,但是对积聚模态和粗模态气溶胶数浓度的影响较小.NPF发生时往往温度较高,风速较大,总辐照度较高,RH较低.NPF天PM2.5、PM10、CO和NO2的浓度较低,O3和SO2浓度较高.40.0%的偏北气团和29.6%的偏南气团可观测到NPF过程.不同气团类型NPF过程中气象要素存在显著差异.南部气团类型NPF过程中风速最小,平均为(2.4±1.5)m·s-1;RH最高,平均为(48.8±10.8)%;北部气团类型NPF过程中风速最大,平均为(4.2±1.9)m·s-1;总辐照度最高,平均为(664.5±255.6)W·m-2;西部气团类型NPF过程中RH最低,平均为(29.8±12.7)%.不同气团类型NPF过程中新粒子的生成速率相差不大,为1.5~1.8cm-3·s-1.南部气团类型NPF过程中增长速率最大,为(12.7±13.6)nm·h-1,是北部气团类型和西部气团类型的1.2倍和1.4倍. 英文摘要 In this study, the aerosol number size distribution in the range of 10 nm-10 μm was collected from August 16 to October 04, 2019 at Ordos using a wide-range particle spectrometer (WPS). Combined with PM (PM2.5 and PM10), pollution gases, meteorological data, and the HYSPLIT model, the characteristics and impact factors of new particle formation (NPF) were discussed. The results indicated that there were 19 NPF events during the observation period, which have different effects on diurnal variation in aerosol number concentration in different modes. The NPF events caused a sharp increase in the number concentration of nucleation and Aitken mode aerosols, but had little effect on the number concentration of accumulation and coarse mode aerosols. The temperature, wind speed, and total solar radiation during NPF days were usually higher than those in non-NPF days, and the RH during NPF days was lower. On NPF days, the mass concentrations of PM2.5, PM10, CO, and NO2 were lower than those on non-NPF days, while the mass concentrations of O3 and SO2 were higher. NPF events were observed in 40.0% of northern air masses and 29.6% of southern air masses. There were significant differences in meteorological elements in different NPF event air mass types. The southern NPF event air mass type had the lowest wind speed and the highest RH, with averages of (2.4±1.5) m·s-1 and (48.8±10.8)%, respectively. The northern NPF event air mass type had the highest wind speed and total solar radiation, with averages of (4.2±1.9) m·s-1 and (664.5±255.6) W·m-2, respectively. The western air mass type of NPF event had the lowest RH, with an average of (29.8±12.7)%. The formation rates of new particles in the different air mass types of NPF events were similar, ranging from 1.5 to 1.8 cm-3·s-1. The largest growth rate was (12.7±13.6) nm·h-1 in the southern NPF event air mass type, which was 1.2 times and 1.4 times higher than the NPF events of northern air masses and western air masses.

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