Zhen, Xiaomei1,2,3,4; Li, Yanfang2,3,4; Tang, Jianhui2,3,6
; Wang, Xinming1; Liu, Lin2,3,4; Zhong, Mingyu5; Tian, Chongguo2,3,6发表期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
2021-06-01
卷号55期号:11页码:7376-7385
关键词brominated flame retardantssource and sinkmulti-box mass balance modelriver dischargeatmospheric depositionBDE 209/DBDPE ratioBohai Sea
DOI10.1021/acs.est.0c08528
通讯作者Tang, Jianhui(jhtang@yic.ac.cn)
英文摘要Both decabromodiphenyl ether (BDE 209) and decabromodiphenyl ethane (DBDPE) are still produced in large quantities in China, especially in the Shandong Province closed to the Bohai Sea (BS). This study conducted a comprehensive investigation of the distribution and budget of brominated flame retardants (BFRs) in the BS. BDE 209 was the predominant BFR in most of the investigated rivers flowing into the BS, although DBDPE exceeded BDE 209 in certain rivers as a result of the replacement of BDE 209 with DBDPE in North China. The spatial distributions of BFRs in the rivers were controlled by the proximity of the BFR manufacturing base and the extent of urbanization. BFRs' spatial distribution in the BS was influenced by a combination of land-based pollution sources, environmental parameters (e.g., suspended particulate matter, particulate organic carbon, and particulate black carbon), and hydrodynamic conditions. The spatial variation trend of BDE 209/DBDPE ratios in various environmental media provided useful information. Vertically, the BDE 209/DBDPE ratio decreased from the seawater surface layer to the sediment, indicating their differential transport in the BS. A multi-box mass balance model and analysis of BDE 209 showed that degradation was the primary sink of BFRs in seawater (similar to 68%) and surface sediment (similar to 72%) in the BS.
资助机构National Natural Science Foundation of China (NSFC); Shandong Province Joint Fund; NSFC; key project of Chinese Academy of Sciences; key deployment project of Centre for Ocean Mega-Science, Chinese Academy of Sciences; seed project of Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences
收录类别SCI
语种英语
关键词[WOS]POLYBROMINATED DIPHENYL ETHERS; HALOGENATED FLAME RETARDANTS; LONG-RANGE TRANSPORT; BOHAI SEA; DECHLORANE PLUS; SPATIAL-DISTRIBUTION; YELLOW SEA; SEASONAL-VARIATION; SURFACE SEDIMENTS; RIVER DELTA
研究领域[WOS]Engineering; Environmental Sciences & Ecology
WOS记录号WOS:000659374200019
引用统计
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/29425
专题中科院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
中科院海岸带环境过程与生态修复重点实验室
通讯作者Tang, Jianhui作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510631, Peoples R China
2.Chinese Acad Sci, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res YIC, Yantai 264003, Peoples R China
3.YICCAS, Shandong Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China
4.Univ Chinese Acad Sci UCAS, Beijing 100049, Peoples R China
5.Yantai Univ, Yantai 264005, Shandong, Peoples R China
6.Chinese Acad Sci, Ctr Ocean Megasci, Qingdao 266071, Peoples R China
推荐引用方式
GB/T 7714Zhen, Xiaomei,Li, Yanfang,Tang, Jianhui,et al. Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2021,55(11):7376-7385.
APAZhen, Xiaomei.,Li, Yanfang.,Tang, Jianhui.,Wang, Xinming.,Liu, Lin.,...&Tian, Chongguo.(2021).Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region.ENVIRONMENTAL SCIENCE & TECHNOLOGY,55(11),7376-7385.
MLAZhen, Xiaomei,et al."Decabromodiphenyl Ether versus Decabromodiphenyl Ethane: Source, Fate, and Influencing Factors in a Coastal Sea Nearing Source Region".ENVIRONMENTAL SCIENCE & TECHNOLOGY 55.11(2021):7376-7385.
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