Liu, Xinghua; Zhang, Haibo
; Luo, Yongming; Zhu, Rongsheng; Wang, Huaizhong; Huang, Baohua发表期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
2020-04-20
卷号714页码:136628
关键词VETERINARY ANTIBIOTICSHUMIC SUBSTANCESTETRACYCLINEADSORPTIONFATECLAYCARBONACIDENVIRONMENTWATER
研究领域Environmental Sciences
DOI10.1016/j.scitotenv.2020.136628
产权排序[Liu, Xinghua; Zhu, Rongsheng; Wang, Huaizhong; Huang, Baohua] Shandong Acad Agr Sci, Key Lab Livestock Dis Control & Breeding, Inst Anim Sci & Vet Med, Jinan 250100, Jinan, Peoples R China; [Zhang, Haibo] Zhejiang A&F Univ, Sch Environm & Resource Sci, Key Lab Soil Contaminat Bioremediat Zhejiang Prov, Hangzhou 311300, Peoples R China; [Luo, Yongming] Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Peoples R China; [Liu, Xinghua; Luo, Yongming] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
通讯作者Zhang, Haibo(hbzhang@zafu.edu.cn); Luo, Yongming(ymluo@issas.ac.cn)
作者部门海岸带环境过程实验室
英文摘要Particulate organic matter (POM) is a fraction of organic matter with dissimilar properties in different soils. POM isolated from soils and sediments (wetland, oil waste field, farmlands and aquaculture pond sediment) was used to study its sorption behavior on the antibiotic oxytetracydine (OTC). Impacts of solution pH, ionic strength and temperature on the OTC sorption were studied. The sorption rates of OTC in POM from wetland (POM-w) and farmland (POM-f1, POM-f2) were rapid during the first 3 h and gradually decreased with reaction time until reaching the equilibrium. Linear sorption occurred from 3 to 12 h in POM from oil waste field land (POM-o) and aquaculture pond sediment ( POM-a). The organic carbon normalized partition coefficient (k(oc)) varied from 215.0 to 4493.6 L kg(-1), and it was nearly 10x higher for the POM-w, POM-f1 and POM-f2 than in the POM-o and POM-a. Sorption of OTC by POM exhibited strong pH dependence. Ionic factors affected OTC sorption in POM-f1, POM-12 and POM-a. The sorption capacity declined >50% in a solution with Ca2+ compared to other ions with similar ionic strength. Sorption thermodynamics showed an entropy increasing and endothermic progress during the OTC sorption in POM, implying a spontaneous sorption process. Several mechanisms were involved in OTC sorption in POM, including hydrogen bonding, cation exchange, hydrophobic partitioning and surface complexation. (C) 2020 Elsevier B.V. All rights reserved.
文章类型Article
资助机构National Natural Science Foundation of ChinaNational Natural Science Foundation of China [41371313, 41771351]; Shandong Key Laboratory of Coastal Environmental Processes, YICCAS [2019SDHADKFJJ09]; Innovation Project of Shandong Academy of Agricultural Sciences [CXGC2018E10]; Zhejiang Provincial Natural Science Foundation of ChinaNatural Science Foundation of Zhejiang Province [LZ19D010001]; Zhejiang Agriculture and Forestry University Research Fund [2017FR021]
收录类别SCI
语种英语
关键词[WOS]VETERINARY ANTIBIOTICS; HUMIC SUBSTANCES; TETRACYCLINE; ADSORPTION; FATE; CLAY; CARBON; ACID; ENVIRONMENT; WATER
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000517760200125
引用统计被引频次：8[WOS][WOS记录][WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/25046
专题中科院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
中科院海岸带环境过程与生态修复重点实验室
作者单位1.Shandong Acad Agr Sci, Key Lab Livestock Dis Control & Breeding, Inst Anim Sci & Vet Med, Jinan 250100, Jinan, Peoples R China;
2.Zhejiang A&F Univ, Sch Environm & Resource Sci, Key Lab Soil Contaminat Bioremediat Zhejiang Prov, Hangzhou 311300, Peoples R China;
3.Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Peoples R China;
4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
推荐引用方式
GB/T 7714Liu, Xinghua,Zhang, Haibo,Luo, Yongming,et al. Sorption of oxytetracycline in particulate organic matter in soils and sediments: Roles of pH, ionic strength and temperature[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2020,714:136628.
APALiu, Xinghua,Zhang, Haibo,Luo, Yongming,Zhu, Rongsheng,Wang, Huaizhong,&Huang, Baohua.(2020).Sorption of oxytetracycline in particulate organic matter in soils and sediments: Roles of pH, ionic strength and temperature.SCIENCE OF THE TOTAL ENVIRONMENT,714,136628.
MLALiu, Xinghua,et al."Sorption of oxytetracycline in particulate organic matter in soils and sediments: Roles of pH, ionic strength and temperature".SCIENCE OF THE TOTAL ENVIRONMENT 714(2020):136628.
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