Lu, Yuxi; Gao, Xuelu
; Song, Jinming; Chen, Chen-Tung Arthur; Chu, Jinling发表期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
2020-05-15
卷号717页码:135265
关键词CROSS-FLOW ULTRAFILTRATIONORGANIC-MATTERCENTRIFUGAL ULTRAFILTRATIONCHEMICAL SPECIATIONNARRAGANSETT BAYAQUATIC COLLOIDSSURFACE WATERSDISSOLVED CUCOMPLEXATIONCOPPER
研究领域Environmental Sciences
DOI10.1016/j.scitotenv.2019.135265
产权排序[Lu, Yuxi; Gao, Xuelu; Chu, Jinling] Chinese Acad Sci, Yantai Inst Coastal Zone Res, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Shandong, Peoples R China; [Lu, Yuxi; Gao, Xuelu; Song, Jinming] Univ Chinese Acad Sci, Beijing 100049, Peoples R China; [Song, Jinming] Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Ecol & Environm Sci, Qingdao 266071, Shandong, Peoples R China; [Song, Jinming] Qingdao Natl Lab Marine Sci & Technol, Funct Lab Marine Ecol & Environm Sci, Qingdao 266237, Shandong, Peoples R China; [Chen, Chen-Tung Arthur] Natl Sun Yat Sen Univ, Dept Oceanog, Kaohsiung 80424, Taiwan
通讯作者Gao, Xuelu(xlgao@yic.ac.cn)
作者部门海岸带信息集成与综合管理实验室
英文摘要The environmental characteristics of colloidal toxic trace metals Cd, Cu and Pb in riverine and estuarine waters collected from two urban rivers of Yantai City in eastern China, the Guangdang and Xin'an Rivers, were investigated using a modified centrifugal ultrafiltration (CUF) method in conjunction with acid extraction and inductively coupled plasma mass spectrometry. The target metals in dissolved pool were divided into four CUF fractions, i.e. <1 kDa, 1-3 kDa, 3-10 kDa and 10 kDa-0.2 mu m, and the results showed that colloidal Cd, Cu and Pb were dominated by 1-10 kDa (1-3 and 3-10 kDa), 1-3 kDa and 10 kDa-0.2 lm fractions, respectively. The coagulation/flocculation of low-molecular-weight (1-10 kDa) colloidal Cd and Cu in the estuaries was obvious and strong, while the enrichment of dissolved Pb in the 10 kDa-0.2 lm fraction may be mainly related to its biogeochemical interactions with Fe-oxides, which is easy to occur in macromolecular colloids. In addition, the actual molecular weight cutoffs (MWCOs) of the three used CUF units with nominal MWCOs of 1, 3 and 10 kDa were determined to be 4.9, 8.5 and 33.9 kDa, respectively, indicating that membrane calibration is essential for explaining the actual fraction of dissolved trace metals and verifying the integrity of ultrafiltration membrane. Overall, the results in this study provide a further understanding of the heterogeneity in biogeochemical features, migration and fate of toxic trace metals in aquatic ecosystems, especially that of the river-sea mixing zone. (C) 2019 Elsevier B.V. All rights reserved.
文章类型Article
资助机构Strategic Priority Research Program of the Chinese Academy of SciencesChinese Academy of Sciences [XDA23050303]; National Natural Science Foundation of ChinaNational Natural Science Foundation of China [41376083]
收录类别SCI
语种英语
关键词[WOS]CROSS-FLOW ULTRAFILTRATION; ORGANIC-MATTER; CENTRIFUGAL ULTRAFILTRATION; CHEMICAL SPECIATION; NARRAGANSETT BAY; AQUATIC COLLOIDS; SURFACE WATERS; DISSOLVED CU; COMPLEXATION; COPPER
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000519994800035
引用统计被引频次：3[WOS][WOS记录][WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/25033
专题中科院海岸带环境过程与生态修复重点实验室_海岸带信息集成与战略规划研究中心
中科院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Shandong, Peoples R China;
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China;
3.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Ecol & Environm Sci, Qingdao 266071, Shandong, Peoples R China;
4.Qingdao Natl Lab Marine Sci & Technol, Funct Lab Marine Ecol & Environm Sci, Qingdao 266237, Shandong, Peoples R China;
5.Natl Sun Yat Sen Univ, Dept Oceanog, Kaohsiung 80424, Taiwan
推荐引用方式
GB/T 7714Lu, Yuxi,Gao, Xuelu,Song, Jinming,et al. Colloidal toxic trace metals in urban riverine and estuarine waters of Yantai City, southern coast of North Yellow Sea[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2020,717:135265.
APALu, Yuxi,Gao, Xuelu,Song, Jinming,Chen, Chen-Tung Arthur,&Chu, Jinling.(2020).Colloidal toxic trace metals in urban riverine and estuarine waters of Yantai City, southern coast of North Yellow Sea.SCIENCE OF THE TOTAL ENVIRONMENT,717,135265.
MLALu, Yuxi,et al."Colloidal toxic trace metals in urban riverine and estuarine waters of Yantai City, southern coast of North Yellow Sea".SCIENCE OF THE TOTAL ENVIRONMENT 717(2020):135265.
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