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--> --> -->It is well known that the level structure of nuclei N=50,51 is dominated by single-particle excitations, even for states with high spin. On the other hand, nuclei with N≥55 exhibit collective behavior [8, 9].
As it si a nearly spherical nucleus with N=51 in the A~90 mass region, the studies of the excited states of 92Nb are of importance for establishing and testing the residual interactions in shell model calculations. Previously, the level structure of 92Nb was mainly investigated by proton and 3He induced reactions [10-13], and the energies of excited states were extended up to 3797 keV by the 88Sr (7Li, 3n)92Nb experiment [14]. Recently, high-spin states of 92Nb were studied in the heavy ion fusion-evaporation reaction 82Se (14N,4n)92Nb [15]. For the middle-low excited states of 92Nb, the information is relatively scarce, and thus it is important to further explore this nucleus experimentally. From the theoretical point of view, 92Nb was studied within the framework of the shell model, and its low-lying levels below Elevel=2287 keV [12] were described by taking the even-even nucleus 88Sr as the inert core, while the valance nucleons occupy the πp1/2, g9/2 and νd5/2 orbitals. Nevertheless, from the theoretical point of view, further study of 92Nb is still necessary.
As a “transitional” nucleus with N=52, the excitation of 93Nb is relative intricate [8]. In an earlier work, 93Nb was studied in the (n, nγ) and (p,2nγ) reactions [16]. The Iπ=3/2- at 1840 keV and Iπ=5/2- at 2013 keV were identified as mixed-symmetry states, which can be viewed as low-energy collective modes where protons and neutrons move uncoupled. High-spin states were studied in the 82Se(16O, p4n)93Nb reaction, with the level schemes up to excitation energy of 11 MeV [17]. An M1 rotational band was reported and showed the characteristics of oblate collective rotational band. The investigation of the level structure of 93Nb can provide additional information for a systematic study of nuclei with N=52.
In this work, the low-lying structure of 92Nb was further studied, and its proposed level scheme was calculated using the shell model code NushellX with SNE valence space, and compared with the experimental results. In addition, two new transitions were observed in 93Nb, as discussed in the following section.
The fusion reaction induced by a weakly-bound projectile at near-barrier energies is complicated due to low breakup threshold [6, 20]. When the projectile completely fuses with the target nucleus without breakup (BU), the process is a direct complete fusion (DCF). When the projectiles breakup, then: 1) if all the fragments fuse with the target nucleus, the process is a sequential complete fusion (SCF); or 2) if only part of the fragments fuse with the target nucleus, the process is an incomplete fusion (ICF) [6]. In addition, when a medium-mass target nucleus is involved, the fusion process can evaporate not only neutrons but also light charged particles including protons and alpha particles. In the present experiment, 92Nb can be produced in a complete fusion of 6Li with the 89Y target nuclei, followed by the 1p2n evaporation channel. As a result, the characteristic γ-rays from 92Nb are in coincidence with protons emitted from the compound nucleus, as shown in Fig. 1(a). In addition, the 92Mo residue from the reaction can only be produced by the CF process. The yield ratio of 92Nb to 92Mo (92Nb/92Mo) in the present experiment is around 0.38, which is larger than given by the statistical evaporation model (around 0.26). Such an increment of the 92Nb/92Mo ratio indicates that the ICF process may contribute to the production of 92Nb. Fig. 1(b) shows the γ-ray spectrum measured in coincidence with deuterons, in which the characteristic gamma rays of 92Nb are clearly visible. It is concluded that 92Nb can also be populated in the ICF process of 6Li, where alpha particles from the breakup of 6Li fuse with the 89Y target nucleus, and simultaneously, the other fragment (deuteron) escapes and is detected. In summary, the 92Nb residue observed in this experiment was populated in the 89Y(6Li, p2n)92Nb and 89Y(α,n)92Nb reactions.
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The 93Nb residue in the present experiment can be produced by the complete fusion of 6Li with 89Y , followed by the 1p1n evaporation channel, as can be seen in the proton gated spectrum shown in Fig. 1(a). The cross-section for alpha particle stripping from 6Li on a 89Y target producing 93Nb is small, and this process can be neglected.
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Eγ /keV | Iγa | Eiπ→Efπ | RADOc | Jiπ→Jfπ |
97* | 8.79(159) | 2213→2116 | 0.71(13) | 9(?)→8(?) |
116 | 15.08(80) | 2203→2087 | 1.40(10) | 11?→9? |
126* | 2.68(23) | 2213→2087 | 1.58(25) | 9(?)→9? |
142 | 3.07(27) | 2087→1945 | 1.63(33) | 9?→7? |
148 | 53.81(280) | 2235→2087 | 0.94(5) | 10?→9? |
171* | 0.49(18) | 2116→1945 | — | 8(?)→7? |
328 | 27.18(151) | 3326→2998 | 1.52(9) | 13+→11+ |
344* | 0.82(12) | 2431→2087 | 0.96(23) | 10→9? |
354 * | 0.66(8) | 4941→4587 | 1.46(37) | 15(?)→(13?) |
364* | 0.43(7) | 4587→4223 | 0.96(30) | (13?)→12(?) |
387* | 3.03(41) | 2600→2213 | 0.96(13) | 10(?)→9(?) |
397* | 0.92(25) | 2600→2203 | 0.94(36) | 10(?)→11? |
458* | 1.92(18) | 2693→2235 | 0.71(15) | 11(?)→10? |
471 | 3.53(25) | 3797→3326 | 0.88(8) | (12+)→13+ |
501 | 12.77(180) | 501→0 | 0.80(11) | 6+→7+ |
606* | Wb | 2693→2087 | — | 11(?)→9(?) |
711 | 23.85(126) | 2998→2287 | 1.80(11) | 11+→9+ |
763 | 39.35(168) | 2998→2235 | 0.95(6) | 11+→10? |
790* | 0.66(11) | 4587→3797 | 1.00(25) | (13?)→(12+) |
795 | 1.78(26) | 2998→2235 | — | 11+→11? |
799* | 2.07(26) | 3797→2998 | — | (12+)→13+ |
897* | 1.67(76) | 4223→3326 | 0.91(16) | 12?→11+ |
907* | 2.29(34) | 3194→2287 | 1.78(49) | 11(+)→9+ |
1144* | 0.19(6) | 4941→3797 | — | 15?→(12+) |
1225* | 1.67(18) | 4223→2998 | 0.95(46) | 12(?)→11+ |
1261* | 4.09(52) | 4587→3326 | 1.51(20) | (13?)→13+ |
1444 | 5.05(62) | 1945→501 | 0.94(12) | 7?→6+ |
1586 | 3.09(45) | 2087→501 | — | 9?→6+ |
1694* | Wb | 3897→2203 | — | →11? |
1945 | 2.74(56) | 1945→0 | 1.37(27) | 7?→7+ |
2087 | 100 | 2087→0 | 1.40(8) | 9?→7+ |
2116* | 12.83(358) | 2116→0 | 0.83(19) | 8(?)→7+ |
2213* | 7.67(170) | 2213→0 | 1.66(67) | 9(?)→7+ |
2287 | 61.98(367) | 2287→0 | 1.66(14) | 9+→7+ |
a The errors of the relative intensity include the fitting and efficiency corrections. Wb The intensities of transitions are too weak. c The errors of the ADO ratios include the fitting and efficiency corrections. |
Table1.Transition energies (Eγ) of 92Nb, relative intensities of γ-rays (Iγ), initial and final states for γ-rays, ADO ratios, initial and final spins of the transitions.
In order to obtain the multipolarity of the newly observed γ-rays, the angular distributions of each γ-ray from the oriented residues (ADO) were analyzed. Assuming that γ1 and γ2 are the cascading transitions in the same nucleus, the ADO ratio of γ1 is deduced by Iγ1(152°)/Iγ1(90°), where Iγ1(152° or 90°) represents the intensity of γ1-rays collected by the detectors at 152° or 90° , and in coincidence with γ2-rays measured by all detectors. By calculating the ADO ratio of γ-rays with known multipolarity in 92Mo, 91Mo, 92Nb, 93Nb, 90Zr, 89Zr produced in the present experiment, typical ADO ratios Iγ(152°)/Iγ(90°) for quadrupole and dipole transitions are around 1.6 and 0.8, respectively, as shown in Fig. 4(a). The spins of the states of 92Nb are assigned tentatively. For the two lower transitions, 97 and 126 keV, the intensity balance rule is used, which supports to some extent the spin assignment of the levels .
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Two new transitions, 504 and 572 keV, are added to the level scheme of 93Nb feeding into the 2180 keV state, as shown in Fig. 5. From the summed spectrum of 689 and 541 keV, shown in Fig. 6, the peaks of the new transitions 504 and 572 keV can be clearly seen. The ADO ratios for the two transitions are 1.45 and 0.94, indicating quadrupole and dipole properties, respectively. Therefore, the spins of the 2752 keV and 2684 keV states are assigned as 21/2, and 19/2, respectively. The relative intensities of partial γ-rays from 93Nb are given in Table 2.
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Eγ/keV | Iγa | E iπ→Efπ | Jiπ→Jfπ |
156 | 8.1(19) | 1491→1335 | 15/2+→17/2+ |
385 | 58.8(69) | 1335→950 | 17/2+→13/2+ |
504 * | 2.8(6) | 2684→2180 | (19/2)→(17/2?) |
541 | 39.9(69) | 1491→950 | 15/2+→13/2+ |
572* | 1.5(5) | 2752→2180 | (21/2)→(17/2?) |
689 | 7.1(21) | 2180→1491 | (17/2?)→15/2+ |
845 | 2.2(3) | 2180→1335 | (17/2?)→17/2+ |
906 | 10.8(24) | 3086→2180 | (21/2)→(17/2?) |
950 | 100 | 950→0 | 13/2+→9/2+ |
1498 | 25.7(36) | 2833→1335 | 25/2(?)→17/2+ |
a The errors on the relative intensity include the fitting and efficiency corrections. |
Table2.Transition energies (Eγ) of 93Nb, relative intensities of γ-rays (Iγ), initial and final spins of the transitions.
In order to study the levels in 92Nb, we performed shell model calculations with the code NushellX. The SNE model space and SNET interaction were adopted, which were previously used for level structures of nearly spherical nuclei 85Br [27], 96Ru [26], 94Mo [8]. The model space includes 8 proton orbitals (1f5/2, 2p3/2, 2p1/2, 1g9/2, 1g7/2, 2d5/2, 2d3/2, 3s1/2) and 9 neutron orbitals (1f5/2, 2p3/2, 2p1/2, 1g9/2, 1g7/2, 2d5/2, 2d3/2, 3s1/2, 1h11/2) relative to the inert 56Ni (Z = 28, N = 28) core.
The low-excited states of 92Nb behave like single particle excitation, and thus we describe the low-excited states of 92Nb as pure configurations, which means that each state corresponds to one proton orbital and one neutron orbital. The pure configuration calculations were also carried out for the low-excited states of 91Zr, 93Mo, 95Ru [28]. Since the Fermi levels of 92Nb lie at the πg9/2 and νd5/2 orbitals, the quasi-magic nucleus 90Zr is taken as the inert core to describe the low-lying states of 92Nb, so that the 1f5/2, 2p3/2, 2p1/2 proton orbitals and the 1f5/2, 2p3/2, 2p1/2, 1g9/2 neutron orbitals are fully occupied. The first six positive parity states of 92Nb (Iπ=2+~7+) have been previously interpreted as the π(1g9/2)
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I π | configuration | Eexp/MeV | Ecal1/MeV |
2+ | πg9/2![]() ![]() | 0.136 | 0.326 |
3+ | 0.286 | 0.402 | |
4+ | 0.480 | 0.495 | |
5+ | 0.357 | 0.372 | |
6+ | 0.501 | 0.515 | |
7+ | 0 | 0 | |
2? | π(p1/2)-1(g9/2)2![]() ![]() | 0.227 | 0.275 |
3? | 0.391 | 0.314 | |
7? | 1.945 | 1.83 | |
8? | 2.116 | 2.028 | |
9?(1) | 2.088 | 1.900 | |
9?(2) | 2.213 | 2.54 | |
10?(1) | 2.235 | 2.203 | |
10?(2) | 2.6 | 2.643 | |
9+ | π(p1/2)-2(g9/2)3![]() ![]() | 2.287 | 2.552 |
11+ | 2.998 | 3.295 | |
12+ | 3.797 | 3.859 | |
13+ | 3.326 | 3.528 | |
1 the result of shell model calculation with pure configurations. |
Table3.Dominant configurations of the low-lying excited states of 92Nb proposed by the shell model calculations with a pure configuration and SNET interaction, calculated results and experimental level energies.
For the higher excited states of 92Nb, 90Zr is not an ideal core anymore, which makes the configuration of the high-excited states more complicated, as the pure configurations cannot describe the high-excited states properly. In order to study the high-excited states of 92Nb, a large-basis shell model calculation is necessary.
To obtain a more appropriate description of the observed high-excited states of 92Nb, large-basis shell model calculations are used. 92Nb has 13 valence protons and 23 valence neutrons outside the 56Ni core. Due to the large number of active orbitals, truncation of the model space is necessary. In the calculations of 92Nb, the valance space is restricted to π(1f5/24-6, 2p3/22-4, 2p1/20-2, 1g9/21-6, 1g7/20-0, 2d5/20-0, 2d3/20-0, 3s1/20-0)
I π | Eexp /MeV | Ecal2/MeV | configuration | partition(%) |
9+ | 2.287 | 2.111 | 6 4 0 3![]() ![]() | 50.24 |
4 4 2 3![]() ![]() | 13.84 | |||
11+ | 2.998 | 3.146 | 6 4 0 3![]() ![]() | 58.88 |
12+ | 3.797 | 3.746 | 6 4 0 3![]() ![]() | 64.89 |
13+ | 3.326 | 3.325 | 6 4 0 3![]() ![]() | 61.88 |
8? | 2.116 | 2.320 | 6 4 0 3![]() ![]() | 38.79 |
6 4 2 1![]() ![]() | 21.59 | |||
9? | 2.088 | 2.232 | 6 4 0 3![]() ![]() | 30.85 |
6 4 2 1![]() ![]() | 12.36 | |||
9?(2) | 2.213 | 2.777 | 6 4 1 2![]() ![]() | 52.03 |
10? | 2.235 | 1.863 | 6 4 0 3![]() ![]() | 41.57 |
10?(2) | 2.6 | 2.841 | 6 4 1 2![]() ![]() | 49.4 |
13? | 4.587 | 4.797 | 6 4 0 3![]() ![]() | 31.97 |
15? | 4.941 | 5.207 | 6 4 0 3![]() ![]() | 65.92 |
2 the result of shell model calculation with mixed configurations. |
Table4.Main partition of the wave function for high-spin states of 92Nb. Each angular momentum is composed of several different partitions. Each partition is of the form p=π[p(1), p(2), p(3), p(4)]
We are grateful to the INFN-LNL staff for providing stable 6Li beam throughout the experiment. This research was also supported by the HIRFL User Project, CAS.