Pan, Xiaohui1; Zhen, Xiaomei1,2,3; Tian, Chongguo1
; Tang, Jianhui1发表期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
2021-01-10
卷号751页码:8
关键词SCCPsMCCPXiaoqing RiverEstuarine turbidity maximum zoneLaizhou BaySourceFate
DOI10.1016/j.scitotenv.2020.141769
通讯作者Tang, Jianhui(jhtang@yic.ac.cn)
英文摘要Chlorinated paraffins (CPs) are widely employed in a variety of domestic and industrial products, and are ubiquitously detected in the environment. Short-chain chlorinated paraffins (SCCPs) have been listed in the Stockholm Convention as persistent organic pollutants (POPs), but not medium-chain chlorinated paraffins (MCCPs), even though they exhibit physicochemical properties and environmental behaviors similar to SCCPs. However, very limited data are available regarding their environmental behaviors and fates in river-estuary systems. China is the major producer of chlorinated paraffins (CPs), and Shandong Province is the main producer of CPs in China. Here, we investigated the distribution, transport, and fate of SCCPs and MCCPs in a heavily polluted river in Shandong Province, aiming to explore the distributions of CPs between dissolved and particulate phases, and between water and sediment phases, as well as the transport of CPs from river headwaters to estuaries and the roles of the estuarine turbidity maximum zone (ETM) on the fate of CPs. CP concentrations in sediments were 9.1-16,000 ng/g dw(mean value: 1000 ng/g dw) for SCCPs and 2.4-27,000 ng/g dw (mean value: 4400 ng/g dw) for MCCPs. In the water column, CP concentrations were 7.4-470 ng/L for SCCPs (mean value: 43 ng/L) and 4.0-120 ng/L for MCCPs (mean value: 27 ng/L). CP concentrations in riverine sediments were among the highest worldwide. SCCPs accounted for 95% of CPs (sum of SCCPs and MCCPs) in the dissolved phase. Cities around the river basin were found to be important pollution sources for CPs. Long-chained and more chlorinated congeners with larger LogKow values might be more likely to be 'salted-out', and thus, will be sequestrated in sediments in the ETM, while those lighter congener groups with relatively high water solubility were prone to be transported by water flow to larger distances. (C) 2020 Elsevier B.V. All rights reserved.
资助机构National Natural Science Foundation of China; Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences; Key deployment project of Centre for Ocean Mega -Science, Chinese Academy of Sciences
收录类别SCI
语种英语
关键词[WOS]LAIZHOU BAY; EMISSION INVENTORY; MARINE-SEDIMENTS; SUBSTANCES; LEGACY; RISKS; BASIN
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000587300800081
引用统计被引频次：4[WOS][WOS记录][WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/28276
专题中科院海岸带环境过程与生态修复重点实验室
中科院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
通讯作者Tang, Jianhui作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Beijing, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714Pan, Xiaohui,Zhen, Xiaomei,Tian, Chongguo,et al. Distributions, transports and fates of short- and medium-chain chlorinated paraffins in a typical river-estuary system[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,751:8.
APAPan, Xiaohui,Zhen, Xiaomei,Tian, Chongguo,&Tang, Jianhui.(2021).Distributions, transports and fates of short- and medium-chain chlorinated paraffins in a typical river-estuary system.SCIENCE OF THE TOTAL ENVIRONMENT,751,8.
MLAPan, Xiaohui,et al."Distributions, transports and fates of short- and medium-chain chlorinated paraffins in a typical river-estuary system".SCIENCE OF THE TOTAL ENVIRONMENT 751(2021):8.
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