Liu, Haitao1,2; Li, Bo3; Qi, Hong3; Ma, Lixin3; Xu, Jianzhong1; Wang, Minling4; Ma, Wenwen5; Tian, Chongguo5
发表期刊ATMOSPHERE
2021-03-01
卷号12期号:3页码:13
关键词polycyclic aromatic hydrocarbonsatmospheresource apportionmenttoxic potencyHarbin
DOI10.3390/atmos12030297
通讯作者Qi, Hong(hongqi@hit.edu.cn)
英文摘要A total of 68 PUF samples were collected seasonally from 17 sampling sites in Harbin, China from May 2016 to April 2017 for analyzing 15 congeners of gaseous polycyclic aromatic hydrocarbons (sigma(15)PAHs). An improved non-negative matrix (NMF) model and a positive matrix factorization (PMF) model were used to apportion the sources of PAHs. The carcinogenic risk due to exposure to PAHs was estimated by the toxicity equivalent of BaP (BaPeq). The results showed that the average concentration of sigma(15)PAHs was 68.3 +/- 22.3 ng/m(3), and the proportions of 3-ring, 4-ring, 5-ring, and 6-ring PAHs were 64.4%, 32.6%, 2.10%, and 0.89%, respectively. Among the six typical functional areas in Harbin, the sigma(15)PAHs concentrations were 98.1 +/- 76.7 ng/m(3), 91.2 +/- 76.2 ng/m(3), 71.4 +/- 75.6 ng/m(3), 67.9 +/- 65.6 ng/m(3), 42.6 +/- 34.7 ng/m(3), and 38.5 +/- 38.0 ng/m(3) in the wastewater treatment plant, industrial zone, business district, residential area, school, and suburb, respectively. During the sampling period, the highest concentration of sigma(15)PAHs was in winter. The improved NMF model and PMF model apportioned the PAHs into three sources including coal combustion, biomass burning, and vehicle exhaust. The contributions of coal combustion, biomass burning, and vehicle exhausts were 34.6 +/- 3.22%, 48.6 +/- 4.03%, and 16.8 +/- 5.06%, respectively. Biomass burning was the largest contributor of sigma(15)PAHs concentrations in winter and coal combustion contributed significantly to the concentrations in summer. The average sigma BaPeq concentration was 0.54 +/- 0.23 ng/m(3) during the sampling period, high concentrations occurred in the cold season and low levels presented in the warm period. Vehicle exhaust was the largest contributor to the sigma BaPeq concentration of PAHs in Harbin.
资助机构National Natural Science Foundation of China; Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences
收录类别SCI
语种英语
研究领域[WOS]Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences
WOS记录号WOS:000633329900001
引用统计被引频次：1[WOS][WOS记录][WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/27333
专题中科院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
中科院海岸带环境过程与生态修复重点实验室
通讯作者Qi, Hong作者单位1.Harbin Engn Univ, Sch Econ & Management, Harbin 150007, Peoples R China
2.Heilongjiang Univ Sci & Technol, Sch Min Engn, Harbin 150022, Peoples R China
3.Harbin Inst Technol, State Key Lab Urban Water Resources & Environm, Harbin 150090, Peoples R China
4.Shandong Prov Yantai Ecol Environm Monitoring Ctr, Yantai 264000, Peoples R China
5.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
推荐引用方式
GB/T 7714Liu, Haitao,Li, Bo,Qi, Hong,et al. Source Apportionment and Toxic Potency of Polycyclic Aromatic Hydrocarbons (PAHs) in the Air of Harbin, a Cold City in Northern China[J]. ATMOSPHERE,2021,12(3):13.
APALiu, Haitao.,Li, Bo.,Qi, Hong.,Ma, Lixin.,Xu, Jianzhong.,...&Tian, Chongguo.(2021).Source Apportionment and Toxic Potency of Polycyclic Aromatic Hydrocarbons (PAHs) in the Air of Harbin, a Cold City in Northern China.ATMOSPHERE,12(3),13.
MLALiu, Haitao,et al."Source Apportionment and Toxic Potency of Polycyclic Aromatic Hydrocarbons (PAHs) in the Air of Harbin, a Cold City in Northern China".ATMOSPHERE 12.3(2021):13.
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