Catalytic conversion of gaseous tars using land, coastal and marine biomass-derived char catalysts i

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Catalytic conversion of gaseous tars using land, coastal and marine biomass-derived char catalysts in a bench-scale downstream combined fixed bed system
Li, Jie

; Liu, Zhengyi

; Tian, Yuanyu ; Zhu, Yanan ; Qin, Song

; Qiao, Yingyun
发表期刊BIORESOURCE TECHNOLOGY

ISSN0960-8524
2020-05
卷号304 页码:122735
关键词RICH GAS-PRODUCTION STEAM GASIFICATION CO-PYROLYSIS MODEL TAR REMOVAL CRACKING SYNGAS DECOMPOSITION TEMPERATURE REACTIVITY
研究领域Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels
DOI10.1016/j.biortech.2020.122735
产权排序[Li, Jie; Tian, Yuanyu; Zhu, Yanan; Qiao, Yingyun] China Univ Petr East China, State Key Lab Heavy Oil Proc, Qingdao 266580, Shandong, Peoples R China; [Li, Jie; Tian, Yuanyu; Qiao, Yingyun] Shandong Univ Sci & Technol, Coll Chem & Environm Engn, Key Lab Low Carbon Energy & Chem Engn, Qingdao 266590, Shandong, Peoples R China; [Liu, Zhengyi; Qin, Song] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264000, Shandong, Peoples R China; [Li, Jie; Tian, Yuanyu; Qiao, Yingyun] Shandong Engn & Technol Res Ctr High Carbon Energ, Qingdao 266590, Shandong, Peoples R China
通讯作者Qiao, Yingyun(qiao_yingyun@126.com)
作者部门海岸带生物学与生物资源保护实验室
英文摘要The catalytic activity of biochar for tar removal was evaluated in a bench-scale combined fixed bed reactor by comparison of gaseous tar catalytic cracking behaviors over land (Corn stalks, Cs), coastal (Reed, Re) and marine (Sargassum horneri, Sh) char catalyst. The experiments demonstrated that the tar yield after addition of the biochar was reduced significantly; the tar conversion efficiency reached to 94.6% for catalytic at 850 degrees C with 50 mm char bed length using Re char. And the yield and composition of gas also changed markedly. The percentage of H-2 and CO in the product gas were obviously increased. Sh has a higher H-2 content (49.3% of the total gas content), whereas, CO dominated in the gas products for Cs (45.4%) and Re (48.1%). The results from GC-MS analysis illustrated that the increase in temperature promoted the tar cracking and also promotes the polymerization of some tar components.
文章类型Article
资助机构National Natural Science Foundation of ChinaNational Natural Science Foundation of China [2157060571, 21576294, 21706287]; Taishan Scholar Foundation of Shandong Province [tsqn201812028]; Department of Science and Technology of Shandong Province [2018CXGC0301]; Qingdao Municipal Science and Technology Bureau [16-6-2-51nsh, 18-6-1-101-nsh]; Fundamental Research Funds for the Central UniversitiesFundamental Research Funds for the Central Universities [18CX05022A]; Independent Innovation Research Project of China University of Petroleum (East China) [YJ201601066]; Postgraduate Innovation Funding Project of China University of Petroleum (East China) [YCX2019033]
收录类别SCI
语种英语
关键词[WOS]RICH GAS-PRODUCTION; STEAM GASIFICATION; CO-PYROLYSIS; MODEL TAR; REMOVAL; CRACKING; SYNGAS; DECOMPOSITION; TEMPERATURE; REACTIVITY
研究领域[WOS]Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels
WOS记录号WOS:000518852900012
引用统计被引频次：11[WOS][WOS记录][WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/25041
专题海岸带生物学与生物资源利用重点实验室_海岸带生物学与生物资源保护实验室

作者单位1.China Univ Petr East China, State Key Lab Heavy Oil Proc, Qingdao 266580, Shandong, Peoples R China;
2.Shandong Univ Sci & Technol, Coll Chem & Environm Engn, Key Lab Low Carbon Energy & Chem Engn, Qingdao 266590, Shandong, Peoples R China;
3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264000, Shandong, Peoples R China;
4.Shandong Engn & Technol Res Ctr High Carbon Energ, Qingdao 266590, Shandong, Peoples R China

推荐引用方式
GB/T 7714Li, Jie,Liu, Zhengyi,Tian, Yuanyu,et al. Catalytic conversion of gaseous tars using land, coastal and marine biomass-derived char catalysts in a bench-scale downstream combined fixed bed system[J]. BIORESOURCE TECHNOLOGY,2020,304:122735.
APALi, Jie,Liu, Zhengyi,Tian, Yuanyu,Zhu, Yanan,Qin, Song,&Qiao, Yingyun.(2020).Catalytic conversion of gaseous tars using land, coastal and marine biomass-derived char catalysts in a bench-scale downstream combined fixed bed system.BIORESOURCE TECHNOLOGY,304,122735.
MLALi, Jie,et al."Catalytic conversion of gaseous tars using land, coastal and marine biomass-derived char catalysts in a bench-scale downstream combined fixed bed system".BIORESOURCE TECHNOLOGY 304(2020):122735.

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