Li, Jia; Zhang, Kaina; Zhang, Hua
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2018-06
卷号237页码:460-467
关键词AntibioticsMicroplasticsAdsorptionDistribution coefficient
研究领域Environmental Sciences & Ecology
DOI10.1016/j.envpol.2018.02.050
产权排序[Li, Jia; Zhang, Hua] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Li, Jia] Univ Chinese Acad Sci, Beijing 100049, Peoples R China; [Zhang, Kaina] YanTai Univ, Sch Environm & Mat Engn, Yantai 264003, Peoples R China
作者部门海岸带环境过程实验室
英文摘要Microplastics and antibiotics are two classes of emerging contaminants with proposed negative impacts to aqueous ecosystems. Adsorption of antibiotics on microplastics may result in their long-range transport and may cause compound combination effects. In this study, we investigated the adsorption of 5 antibiotics [sulfadiazine (SDZ), amoxicillin (AMX), tetracycline (TC), ciprofloxacin (CIP), and trimethoprim (TMP)] on 5 types of microplastics [polyethylene (PE), polystyrene (PS), polypropylene (PP), polyamide (PA), and polyvinyl chloride (PVC)] in the freshwater and seawater systems. Scanning Electron Microscope (SEM) and X-ray diffractometer (XRD) analysis revealed that microplastics have different surface characterizes and various degrees of crystalline. Adsorption isotherms demonstrated that PA had the strongest adsorption capacity for antibiotics with distribution coefficient (K-d) values ranged from 7.36 +/- 0.257 to 756 +/- 48.0 L kg(-1) in the freshwater system, which can be attributed to its porous structure and hydrogen bonding. Relatively low adsorption capacity was observed on other four microplastics. The adsorption amounts of 5 antibiotics on PS, PE, PP, and PVC decreased in the order of CIP > AMX > TMP > SDZ > TC with K-f correlated positively with octanol-water partition coefficients (Log K-OW). Comparing to freshwater system, adsorption capacity in seawater decreased significantly and no adsorption was observed for CIP and AMX. Our results indicated that commonly observed polyamide particles can serve as a carrier of antibiotics in the aquatic environment. (C) 2018 Elsevier Ltd. All rights reserved.
文章类型Article
资助机构National Key R D projects [2016YFC1402202]; Key projects of international cooperation of Chinese Academy of Sciences [KYSB20160003]
收录类别SCI
语种英语
关键词[WOS]PERSISTENT ORGANIC POLLUTANTS; MARINE-ENVIRONMENT; HUMIC SUBSTANCES; WASTE-WATER; SORPTION; CHINA; PHARMACEUTICALS; RESISTANCE; RIVER; TRANSPORT
研究领域[WOS]Environmental Sciences
WOS记录号WOS:000431158900047
引用统计被引频次：327[WOS][WOS记录][WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cnhttp://ir.yic.ac.cn/handle/133337/24457
专题中科院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
中科院海岸带环境过程与生态修复重点实验室_污染过程与控制实验室
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China;
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China;
3.YanTai Univ, Sch Environm & Mat Engn, Yantai 264003, Peoples R China
推荐引用方式
GB/T 7714Li, Jia,Zhang, Kaina,Zhang, Hua. Adsorption of antibiotics on microplastics[J]. ENVIRONMENTAL POLLUTION,2018,237:460-467.
APALi, Jia,Zhang, Kaina,&Zhang, Hua.(2018).Adsorption of antibiotics on microplastics.ENVIRONMENTAL POLLUTION,237,460-467.
MLALi, Jia,et al."Adsorption of antibiotics on microplastics".ENVIRONMENTAL POLLUTION 237(2018):460-467.
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