个人简介
张光辉，博士，副教授，硕士生导师，大连理工大学第三批“星海青千”。2007年毕业于南京师范大学化学专业获学士学位；2010年毕业于南京师范大学有机化学专业孙培培教授课题组获硕士学位；2014年毕业于武汉大学有机化学专业雷爱文教授课题组获得博士学位。攻读博士学位期间曾于2012年-2014年在美国阿贡国家实验室合作研究。获得博士学位之后，曾先后在美国伊利诺伊理工学院化学系/阿贡国家实验室Adam S. Hock教授课题组（2014-2016年）、普渡大学化工系Jeffrey T. Miller教授课题组（2016-2018年）任博士后研究员，并于2018年加入大连理工大学化工学院。近年来主要利用原位光谱学方法研究催化反应机理，探讨催化剂活性中心的结构与反应活性之间的构效关系，在均相催化、多相催化领域都有丰富的研究经验和基础。相关研究结果建立了若干催化反应中催化活性位点与催化反应活性之间的构效关系，为新型催化剂的设计、合成提供了重要的理论依据和指导。在页岩气催化转化领域的研究方面也有重要的发现，发展了一系列新型高效的页岩气转化双金属及单原子催化剂，为提高页岩气资源的高效利用提供了新的突破。在化学、催化领域内的国际期刊上发表SCI论文70余篇，Wiley书籍1章。据Web of Science统计，论文被引1000余次，个人H因子为22。
https://orcid.org/0000-0002-5854-6909
https://publons.com/researcher/**/guanghui-zhang/
张光辉博士目前的研究兴趣主要集中在多相催化领域，尤其是二氧化碳、烷烃等小分子的催化转化。2019年起招收研究生，欢迎具有化学、化工、材料背景，对纳米材料、多相催化、表面金属有机化学、催化剂原位表征感兴趣的同学报考。
联系方式：gzhang@dlut.edu.cn
Dr. Guanghui Zhang is an associate professor of chemical engineering at Dalian University of Technology. He obtained his B.S. in chemistry and M.S. in organic chemistry from Nanjing Normal University in 2007 and 2010, respectively. He received his PhD in chemistry at Wuhan University in 2014 (Prof. Aiwen Lei's group). From 2012 to 2014, he was a visiting graduate student at Argonne National Laboratory. In 2014, he joined Prof. Adam S. Hock's group at Illinois Institute of Technology/Argonne National Laboratory as a senior research associate, and in 2016, he moved to Purdue University working with Prof. Jeffrey T. Miller. He joined Dalian University of Technology in 2018.His research interest lies in heterogeneous catalysis, homogeneous catalysis, organometallic chemistry, and synchrotron-related X-ray spectroscopy. His current research focuses on the development of new catalytic materials for energy and environmental applications.
Selected Recent Publications
Wan, G.; Zhang, G.; Lin, X.-M.: Toward Efficient Carbon and Water Cycles: Emerging Opportunities with Single-Site Catalysts Made of 3d Transition Metals. Adv. Mater. 2020, 32, ** (corresponding author)
Wang, J.; Liu, C.-Y.; Senftle, T.P.; Zhu, J.; Zhang, G.; Guo, X.; Song, C.: Variation in In2O3 Crystal Phase Alters Catalytic Performance toward the Reverse Water Gas Shift Reaction. ACS Catal. 2020, 10,3264?3273 (corresponding author, cover)
Zhang, X.; Han, S.; Zhu, B.; Zhang, G.; Li, X.; Gao, Y.; Wu, Z.; Yang, B.; Liu, Y.; Baaziz, W.; Ersen, O.; Gu, M.; Miller, J.T.; Liu, W.: Reversible Loss of Core-shell Structure for Ni-Au Bimetallic Nanoparticles During CO2 Hydrogenation. Nat. Catal.2020, DOI: 10.1038/s41929-020-0440-2(co-first author)
Zhang, G.; Ye, C.; Liu, W.; Zhang, X.; Yang, X.; Zhu Chen, J.; Wu, Z.; Miller, J. T.: Diffusion Limited Formation of Non-Equilibrium Intermetallic Nanophase for Selective Dehydrogenation. Nano Lett. 2019, 19, 4380-4383
Cesar, L.G.; Yang, C.; Lu, Z.; Ren, Y.; Zhang, G.; Miller, J.T.:Identification of a Pt3Co Surface Intermetallic Alloy in Pt-Co Propane Dehydrogenation Catalysts. ACS Catal. 2019, 9, 5231-5244 (corresponding author)
LiBretto, N.J.; Yang, C.; Ren, Y.;Zhang, G.; Miller, J.T.:Identification of Surface Structures in Pt3Cr Intermetallic Nanocatalysts.Chem. Mater.2019, 31, 1597-1609 (corresponding author)
Wu, Z.; Bukowski, B. C.; Li, Z.; Milligan, C.; Zhou, L.; Ma, T.; Wu, Y.; Ren, Y.; Ribeiro, F. H.; Delgass, W. N.; Greeley, J.; Zhang, G.; Miller, J. T.: Changes in Catalytic and Adsorptive Properties of 2 nm Pt3Mn Nanoparticles by Subsurface Atoms. J. Am. Chem. Soc. 2018, 140, 14870-14877 (corresponding author)
Shen, X.; Zhang, C.; Zhang, S.; Dai, S.; Zhang, G.; Ge, M.; Pan, Y.; Sharkey, S.; Graham, G.; Hunt, A.; Waluyo, I.; Miller, J. T.; Pan, X.; Peng, Z.: Deconvolution of octahedral Pt3Ni nanoparticle growth pathway from in situ characterizations. Nat. Commun.2018, 9. 4485 (co-first author)
Ye, C.; Wu, Z; Liu, W.; Ren, Y.; Zhang, G.; Miller, J.T.: Structure Determination of a Surface Tetragonal Pt1Sb1 Phase on Pt Nanoparticles. Chem. Mater. 2018, 30, 4503-4507 (corresponding author)
An, S.; Zhang, G.; Wang, T.; Zhang, W.; Li, K.; Song, C.; Miller, J.T.; Miao, S.; Wang, J; Guo, X.: High-Density Untrasmall Cluster and Single-atom Fe Sites Embedded in g-C3N4 for Highly Efficient Catalytic Advanced Oxidation Processes. ACS Nano 2018, 12, 9441-9450 (co-first author)
Zhang, G.; Yi, H.; Zhang, G. T.; Deng, Y.; Bai, R. P.; Zhang, H.; Miller, J. T.; Kropf, A. J.; Bunel, E. E.; Lei, A. W.: Direct Observation of Reduction of Cu(II) to Cu(I) by Terminal Alkynes. J. Am. Chem. Soc. 2014, 136, 924-926.
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研究领域
工业催化、能源与环境催化、金属有机催化、催化剂原位表征论文成果
Zeng, Zhenxing,Zhang, Shushen,Su, Yan,Quan, Xie,Choi, Wonyong,Zhang, Guanghui,Liu, Ning,Kim, Bupmo,Chen, Shuo,Yu, Hongtao.Single-atom platinum confined by the interlayer nanospace of carbon nitride for efficient photocatalytic hydrogen evolution[J],NANO ENERGY,2020,69 Wan, Gang,Zhang, Guanghui,Lin, Xiao-Min.Toward Efficient Carbon and Water Cycles: Emerging Opportunities with Single-Site Catalysts Made of 3d Transition Metals[J],ADVANCED MATERIALS,2020,32(2):e**
Zhang, Guanghui,Ye, Chenliang,Liu, Wei,Zhang, Xiaoben,Su, Dangsheng,Yang, Xin,Chen, Johnny Zhu,Wu, Zhenwei,Miller, Jeffrey T..Diffusion-Limited Formation of Nonequilibrium Intermetallic Nanophase for Selective Dehydrogenation[J],NANO LETTERS,2019,19(7):4380-4383
Chen, Johnny Zhu,Wu, Zhenwei,Zhang, Xiaoben,Choi, Slgi,Xiao, Yang,Varma, Arvind,Liu, Wei,Zhang, Guanghui,Miller, Jeffrey T..Identification of the structure of the Bi promoted Pt non-oxidative coupling of methane catalyst: a nanoscale Pt3Bi intermetallic alloy[J],CATALYSIS SCIENCE & TECHNOLOGY,2019,9(6):1349-1356
Liu, Junhui,Zhang, Anfeng,Jiang, Xiao,Zhang, Guanghui,Sun, Yanwei,Liu, Min,Ding, Fanshu,Song, Chunshan,Guo, Xinwen.Overcoating the Surface of Fe-Based Catalyst with ZnO and Nitrogen-Doped Carbon toward High Selectivity of Light Olefins in CO2 Hydrogenation[J],INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2019,58(10):4017-4023
Cesar, Laryssa Goncalves,Yang, Ce,Lu, Zheng,Ren, Yang,Zhang, Guanghui,Miller, Jeffrey T..Identification of a Pt3Co Surface Intermetallic Alloy in Pt-Co Propane Dehydrogenation Catalysts[J],ACS CATALYSIS,2019,9(6):5231-5244
李文慧,张光辉,Xiao Jiang,刘怡,朱杰,丁凡舒,刘中民,郭新闻,宋春山.CO2 Hydrogenation on Unpromoted and M-Promoted Co/TiO2 Catalysts (M = Zr, K, Cs): Effects of Crystal Phase of Supports and Metal–Support Interaction on Tuning Product Distribution[J],ACS Catalysis,2019,9:2739-2751
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铂基双金属纳米催化剂用于二氧化碳氧化丙烷脱氢反应研究, 国家自然科学基金项目, 2019/08/16, 进行 Pt@ZSM-48/50的设计合成及其与n-C7异构化反应的构效关系研究, 企事业单位委托科技项目, 2019/06/28-2020/12/28, 进行
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当前位置: 中文主页 >> 科学研究 >> 研究领域工业催化、能源与环境催化、金属有机催化、催化剂原位表征
论文成果
当前位置: 中文主页 >> 科学研究 >> 论文成果[1] Zeng, Zhenxing,Zhang, Shushen,Su, Yan,Quan, Xie,Choi, Wonyong,Zhang, Guanghui,Liu, Ning,Kim, Bupmo,Chen, Shuo,Yu, Hongtao.Single-atom platinum confined by the interlayer nanospace of carbon nitride for efficient photocatalytic hydrogen evolution[J],NANO ENERGY,2020,69
[2] Wan, Gang,Zhang, Guanghui,Lin, Xiao-Min.Toward Efficient Carbon and Water Cycles: Emerging Opportunities with Single-Site Catalysts Made of 3d Transition Metals[J],ADVANCED MATERIALS,2020,32(2):e**
[3] Zhang, Guanghui,Ye, Chenliang,Liu, Wei,Zhang, Xiaoben,Su, Dangsheng,Yang, Xin,Chen, Johnny Zhu,Wu, Zhenwei,Miller, Jeffrey T..Diffusion-Limited Formation of Nonequilibrium Intermetallic Nanophase for Selective Dehydrogenation[J],NANO LETTERS,2019,19(7):4380-4383
[4] Chen, Johnny Zhu,Wu, Zhenwei,Zhang, Xiaoben,Choi, Slgi,Xiao, Yang,Varma, Arvind,Liu, Wei,Zhang, Guanghui,Miller, Jeffrey T..Identification of the structure of the Bi promoted Pt non-oxidative coupling of methane catalyst: a nanoscale Pt3Bi intermetallic alloy[J],CATALYSIS SCIENCE & TECHNOLOGY,2019,9(6):1349-1356
[5] Liu, Junhui,Zhang, Anfeng,Jiang, Xiao,Zhang, Guanghui,Sun, Yanwei,Liu, Min,Ding, Fanshu,Song, Chunshan,Guo, Xinwen.Overcoating the Surface of Fe-Based Catalyst with ZnO and Nitrogen-Doped Carbon toward High Selectivity of Light Olefins in CO2 Hydrogenation[J],INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2019,58(10):4017-4023
[6] Cesar, Laryssa Goncalves,Yang, Ce,Lu, Zheng,Ren, Yang,Zhang, Guanghui,Miller, Jeffrey T..Identification of a Pt3Co Surface Intermetallic Alloy in Pt-Co Propane Dehydrogenation Catalysts[J],ACS CATALYSIS,2019,9(6):5231-5244
[7] 李文慧,张光辉,Xiao Jiang,刘怡,朱杰,丁凡舒,刘中民,郭新闻,宋春山.CO2 Hydrogenation on Unpromoted and M-Promoted Co/TiO2 Catalysts (M = Zr, K, Cs): Effects of Crystal Phase of Supports and Metal–Support Interaction on Tuning Product Distribution[J],ACS Catalysis,2019,9:2739-2751
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当前位置: 中文主页 >> 科学研究 >> 科研项目[1]铂基双金属纳米催化剂用于二氧化碳氧化丙烷脱氢反应研究, 国家自然科学基金, 2019-08-16, 进行
[2]Pt@ZSM-48/50的设计合成及其与n-C7异构化反应的构效关系研究, 2019-06-28-2020-12-28, 进行
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