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--> --> -->There are extensive previously published elastic transfer studies including 14N(10B,14N)10B. The elastic scattering for the 14N+10B system was measured at the energies of 38.1–50.0 MeV [2], 73.9 MeV, and 93.6 MeV [8]. In Ref. [8] the angular distributions of 14N elastically scattered by 10B were measured in the limited angular range of up to 50° in the center of the mass system. In Ref. [2], measurements of angular distributions were extended to large angles (~ 150°) where a significant rise was exhibited. This rise was reproduced by taking into consideration the effect of α-cluster transfer.
In the present work, elastic scattering in the 14N + 10B system was measured at Elab = 21.0 and 24.5 MeV in order to verify the role of α-cluster transfer between 14N and 10B at energies closer to the Coulomb barrier. The interest in such a study is because the number of reaction channels in the scattering decreases rapidly around the Coulomb barrier. The available data [2, 8] for the 14N+10B system were also reanalyzed using both the optical model (OM) and the DWBA method to obtain an energy-dependent potential that could fairly reproduce the elastic scattering data in the full angular range by taking into account the contribution of the α-transfer mechanism.
This work complements the ongoing program for studying elastic scattering at low energies at the DC-60 cyclotron [5, 9], in which scattering in the collision of light heavy ions is studied to take into account the possible contribution of the particle exchange mechanism. The paper is organized as follows. In Section 2, the measurement procedure of 14N +10B angular distribution is described. Section 3 is devoted to theoretical analysis, results, and discussion. A summary is given in Section 4.
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The angular distributions of elastic scattering of 14N on 10B nucleus at the energies of 21.0 MeV and 24.5 MeV are shown in Fig. 2. These distributions were normalized to OM cross sections at small angles, where it is relatively independent of the parameters of the nuclear potential. The normalization error was smaller than 10%. As can be seen from Fig. 2, in the front hemisphere, a smooth decrease in the cross sections is observed without a pronounced oscillation structure. With a further increase in the angles, the decrease stops and a weakly expressed diffraction structure appears with cross sections rising at angles greater than 120°. We estimated the systematic error of measured cross sections to be no larger than 10%. The statistical error was 1%–5% during our measurements in the forward hemisphere region. It increased at large angles, but nowhere did it exceed 10%. The error bars in Fig. 2 are smaller than the size of the experimental points.
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$\begin{split} U{\rm{(}}R{\rm{)}} =& {V_C}(R) - {\rm{ }}{V_0}{\left[ {1 + \exp \left( {\frac{{r - {R_V}}}{{{a_V}}}} \right)} \right]^{ - 1}} \\&- {\rm i}{W_0}{\left[ {1 + \exp \left( {\frac{{r - {R_W}}}{{{a_W}}}} \right)} \right]^{ - 1}}, \end{split}$ ![]() | (1) |
Angular distributions at energies of 24.5–50.0 MeV showed a significant increase in differential cross sections at backward angles, which was assumed to arise from the contribution of α-cluster transfer between 14N and 10B. The experimental data at 21.0 MeV, which is closer to the Coulomb barrier energy for the 14N+10B nuclear system, only showed a slight increase in cross sections at backward angles. However, a rise is already observed at energy 24.5 MeV, confirming that the transfer phenomenon is highly dependent on the projectile’s energy. The angular distributions at the two higher energies 73.92 and 93.6 MeV were measured in a limited angular range and did not extend beyond ~ 50°, and thus, the transfer phenomenon is not presented.
As mentioned above, experimental data in the energy range 21–50 MeV showed a significant increase in cross sections at backward angles, except at Elab=21.0 MeV, which showed a slight increase. Such increase in cross sections could not be reproduced by the simple OM, and its origin was investigated in terms of α-cluster transfer implemented through the distorted waves Born approximation (DWBA) method. As the ground state spin-parity of 14N is Jπ=1+, an alpha particle coupled to a 10B core with Jπ=3+ can be found in two differential orbitals with angular momentum L=2 or L=4. The configuration with the higher angular momentum should be favored as the cluster configuration with L=4 has a theoretical spectroscopic factor much larger than that of the one with L=2 (SA2=0.11 and SA4=0.83) [10]. However, two possible configurations have been taken into account. The experimental angular distributions at the different energies were analyzed up to angles 90° by the optical model to exclude the effect of cluster transfer and other effects that could affect the cross sections at backward angles using the FRESCO code [11]. The comparisons between the experimental angular distributions in the energy range 21–93.6 MeV and theoretical calculations using both OM and DWBA, incorporated in the Coupled Reactions Channels program (FRESCO) [11], are shown in Figs. 3-5 with the potential parameters listed in Table 1.
E/MeV | Model | V0/MeV | W0/MeV | aW/fm | χ2/N | SA | σR/mb |
21.0 | OM | 98.02±5.0 | 14.39±0.7 | 0.39 | 0.18 | 623.4±30 | |
DWBA – L=2 | 0.21 | 0.69±0.04 | |||||
DWBA – L=4 | 0.47 | 0.93±0.04 | |||||
24.5 | OM | 99.33±5.0 | 14.51±0.7 | 0.44 | 0.57 | 789.4±39 | |
DWBA – L=2 | 1.25 | 0.42±0.04 | |||||
DWBA – L=4 | 2.4 | 0.77±0.04 | |||||
38.1 | OM | 87.24±4.3 | 17.0±0.8 | 0.45 | 5.8 | 1121±56 | |
DWBA – L=2 | 18.6 | 0.61±0.033 | |||||
DWBA – L=4 | 7.9 | 0.8±0.033 | |||||
42.0 | OM | 86.8±4.3 | 18.0±0.9 | 0.476 | 6.54 | 1198±60 | |
DWBA – L=2 | 42.2 | 0.62±0.02 | |||||
DWBA – L=4 | 23.6 | 0.78±0.02 | |||||
46.0 | OM | 84.35±4.2 | 22.0±1.1 | 0.402 | 4.3 | 1173±60 | |
DWBA – L=2 | 14.3 | 0.59± 0.03 | |||||
DWBA – L=4 | 6.7 | 0.76± 0.03 | |||||
50.0 | OM | 83.15±4.2 | 23.0±1.2 | 0.393 | 9.3 | 1197±60 | |
DWBA – L=2 | 17.5 | 0.56±0.03 | |||||
DWBA – L=4 | 15.5 | 0.81±0.03 | |||||
73.9 | OM | 76±3.8 | 28.0±1.4 | 0.373 | 4.3 | 1288±60 | |
93.6 | OM | 64±3.2 | 33.0±1.6 | 0.358 | 11.3 | 1313±60 |
Table1.Optical potential parameters for the 14N+10B system at different energies, together with spectroscopic amplitudes extracted from the DWBA analysis. Note that χ2/N values (normalized per number of experimental points) refer to θc.m.<90° for the elastic scattering and the full angular range for the DWBA calculations. The parametersrV, rW, and aV were fixed at 0.92, 1.29, and 0.77 fm, respectively.
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The significant increase in differential cross sections at large angles can be explained as arising from α-cluster transfer as shown by DWBA calculations that were performed to explore this possibility. In this case, the exchange of the α-cluster between the two interacting nuclei 14N, to be treated as (10B – Core) + (α-particle – valence), leads to an exit channel that is physically indistinguishable from the entrance channel. Therefore, the differential cross section is the square of the sum of amplitudes from the pure elastic scattering and the exchange mechanism of the cluster transfer, as follows [12, 13]:
$ \frac{{{\rm d}{\sigma _{el}}}}{{{\rm d}\Omega }} = {\left| {{f_{el}}\left( \theta \right) + {{\rm e}^{{\rm i}\alpha }}S{f_{\rm DWBA}}\left( {\pi - \theta } \right)} \right|^2}, $ ![]() | (2) |
Calculations of transfer are performed using the optical potential parameters obtained from fitting the data in the forward hemisphere up to 90°. The bound state wave function for the relative motion of the α-particle and 10B in the 14N configuration cluster plus core is defined by a Woods-Saxon potential with fixed radius
$ 2(N - 1) + L = \sum\limits_{i = 1}^n {2({n_i}} - 1) + {l_i}, $ ![]() | (3) |
Overlap | N(Number of nodes) | L | S | J = L+S | Binding energy/MeV |
![]() ![]() | 2 | 2 | 0 | 2 | 11.612 |
1 | 4 | 0 | 4 |
Table2.Cluster quantum numbers for the overlaps used in our calculations.
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As can be seen from Figs. 3 and 4 and Table 1, the values of dσ/dσRU at the largest angles (dσ/dσRU~0.2) and the spectroscopic amplitudes are practically independent of the beam energy. The same result was obtained in Ref. [2].
The contribution of the α-cluster in forming the cross sections at backward angles at E = 46.0 MeV, measured by Takai et al. [2], was analyzed within the framework of the DWBA method by code LOLA [15]. Their and our analyses are compatible at the forward angles region, but there is a significant difference at the backward angles, as shown in Fig. 8. However, in Ref. [2], they did not present χ2/N when comparing both theoretical calculations. However, it is clearly shown in Fig. 8 that the current analysis is much better. Our analysis at 46.0 MeV could reproduce the experimental data well, especially at angles > 160°, whereas in the previous analysis the data and the calculations are completely out of phase at large angles (> 160°). It is noteworthy that the extracted SA4 at E = 46.0 MeV from the current work (0.76) is so close to the used SA4 (0.806) in Ref. [2].
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As mentioned before, the investigation of the 10B(14N,10B)14N α-cluster transfer process to L=2 and L=4 orbitals individually leads to an extracted SA4 value of “0.81 ± 0.12”, which is close to the theoretical value calculated by Kurath [10], whereas the extracted SA2 exceeds the theoretical value. Therefore, further calculations were performed to study the 10B(14N,10B)14N α-cluster transfer process by taking into consideration the transfer to L=2 and L=4 orbitals simultaneously. The potential parameters listed in Table 1 are used in the theoretical calculations. The optimal SA2 and SA4 values were searched using the SFRESCO search code [11]. During the search process, SA2 and SA4 were allowed to be changed freely in the range 0.05–0.7 and 0.6–0.95, respectively, till the best agreement between experimental data and calculations was reached. The starting parameters for SA2 and SA4 are 0.1 and 0.83, respectively; these values are adopted from the work of Kurath [10]. The optimal extracted values for SA2 and SA4,as well as the χ2 / N values, at different concerned energies using this technique are listed in Table 3. The comparison between the experimental data and the theoretical calculations using this method are shown in Figs. 9 and 10. Although in an elastic transfer process the entrance and exit channels are identical and consequently the same SA should be taken for both channels, in this case the value of SA2 was used as the spectroscopic amplitude for the entrance channel and the value of SA4 was used as the spectroscopic amplitude for the exit channel. Thus, the experimental differential cross sections
E/MeV | SA2 | SA4 | χ2/N |
21.0 | 0.7±0.11 | 0.81±0.02 | 0.26 |
24.5 | 0.2±0.04 | 0.65±0.01 | 2.3 |
38.1 | 0.54±0.01 | 0.75±0.02 | 10.9 |
42.0 | 0.47±0.01 | 0.81±0.02 | 31.7 |
46.0 | 0.57±0.01 | 0.79±0.01 | 17.3 |
50.0 | 0.5±0.01 | 0.65±0.01 | 15.4 |
Table3.Optimal extracted values for SA2 and SA4 at the different energies (E), taking into account the contribution from L=2 and L=4 orbitals simultaneously as well as the χ2/N values.
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$ {\left( {\frac{{{\rm d}\sigma }}{{{\rm d}\Omega }}} \right)_{{\rm{exp}}}} = {\left( {\frac{{{\rm d}\sigma }}{{{\rm d}\Omega }}} \right)_{{\rm{DWBA (}}L = {\rm{2)}}}} + {\left( {\frac{{{\rm d}\sigma }}{{{\rm d}\Omega }}} \right)_{{\rm{DWBA (}}L = 4{\rm{)}}}}. $ ![]() | (4) |
Figure 11 shows the energy dependence of the found by us potentials, which are listed in Table 1. It is seen that a linear function is a fair approximation for the energy dependence for the depths of the real and imaginary parts of the optical potentials in the energy range from 20 to 100 MeV for the 10B+14N system. With increasing energy, the depth of the real potential decreases and can be approximated by the formula V0 = 107.2-0.46E, and the depth of the imaginary potential increases and is well described by the formula W0 = 8.19+0.268E.
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An important and useful characteristic of optical potentials is the volume integrals over V(r) and W(r),
$ {J}_{V}=\frac{1}{{A}_{p}{A}_{t}}\int V\left(r\right)4\pi {r}^{2}{\rm d}r \;\;\;\;{\rm{and}}\;\;\;\;{J}_{W}=\frac{1}{{A}_{p}{A}_{t}}\int W\left(r\right)4\pi {r}^{2}{\rm d}r. $ ![]() | (5) |
The volume integrals corresponding to the found potentials, as well as the depths, smoothly vary depending on the energy within 200–300 MeV fm3 for JV and 70–210 MeV fm3 for JW. This is consistent with similar dependencies known from the scattering of p + 12С, 3He + 12С, α + 12С, and 12С + 12С [18-20]. Our potentials are physically reasonable, as their volume integrals (JV) are close to that calculated by microscopic models [18].
The energy dependence of the total reaction cross sections σR obtained in this work is presented in Fig. 12. It can be seen that the rapid growth of cross sections at energies in the range of 20–40 MeV is replaced by a slower one at Е greater than 50 MeV.
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It is well known that the total reaction cross section calculated in the framework of the optical model is practically independent of the details of the real part of the optical potential and is mainly determined by the parameters of its imaginary part, the depth of which, as can be seen from Table 1, increases from 14 to 33 MeV with increasing energy up to 93 MeV. The calculated energy dependence of the total cross sections is adequately approximated by the expression:
${{\sigma }_{R}}(E)=1.3 \pi {{\left( A_{P}^{{}^{1}\!\!\diagup\!\!{}_{3}\;}+A_{T}^{{}^{1}\!\!\diagup\!\!{}_{3}\;} \right)}^{2}}\left( 15.97-\frac{12.25}{E}-\frac{3595.1}{{{E}^{2}}} \right).$ ![]() | (6) |
It is shown that the obtained values of the depths of the real and imaginary potentials linearly depend on energy in the energy range from 20 to 100 MeV.
A. A. Ibraheem extends his appreciation to the Deanship of Scientific Research at King Khalid University for funding this work through the research groups program under grant number G.R.P-56-41.